{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1050299306989168768.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"HDL","@value":"http://hdl.handle.net/10228/0002000374"}},{"identifier":{"@type":"URI","@value":"https://kyutech.repo.nii.ac.jp/records/2000374"}},{"identifier":{"@type":"DOI","@value":"10.1016/j.apcata.2022.118539"}},{"identifier":{"@type":"URI","@value":"https://api.elsevier.com/content/article/PII:S0926860X2200062X?httpAccept=text/xml"}},{"identifier":{"@type":"URI","@value":"https://api.elsevier.com/content/article/PII:S0926860X2200062X?httpAccept=text/plain"}}],"resourceType":"学術雑誌論文(journal article)","dc:title":[{"@language":"en","@value":"Fe(III)-Pt(II) oxide-co-sensitized brookite TiO2 nanorods for photocatalytic degradation of acetaldehyde under visible light"}],"dcterms:alternative":[{"@language":"en","@value":"Fe(III)-Pt(II) oxide-co-sensitized brookite TiO<inf>2</inf> nanorods for photocatalytic degradation of acetaldehyde under visible light"}],"dc:language":"en","description":[{"type":"Abstract","notation":[{"@language":"en","@value":"Platinum is widely investigated as co-catalysts for photocatalytic degradation of volatile organic compounds but studies seldom focus on their visible light sensitizing properties. Herein, Pt sensitizers of different oxidation states (0, II, IV) were modified on brookite TiO2 nanorods and investigated for acetaldehyde degradation under visible light. Pt(II) oxide/TiO2 showed the best photocatalytic activity but its stability was compromised by its self-oxidation to Pt(IV) during photo-oxidation reaction. Surface modification of an Fe(III) oxide thin film sensitizer layer around the Pt(II) oxide sensitizer was found to enhance both the stability and activity of Pt(II) oxide/TiO2. In situ double beam photoacoustic spectroscopy (DB-PAS) supported by DFT modeling showed the rapid injection of photoexcited electrons from Fe(III) oxide to Pt(II) oxide promote the stability of Pt(II) oxide, leading to enhanced performance. The findings provide guidance for the rational design of visible light-active metal oxide sensitizers for oxidative removal of indoor air pollutants."}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1070299306989168770","@type":"Researcher","foaf:name":[{"@language":"en","@value":"Cao, Yu"}]},{"@id":"https://cir.nii.ac.jp/crid/1070299306989168642","@type":"Researcher","foaf:name":[{"@language":"en","@value":"Lou, Shi Nee"}]},{"@id":"https://cir.nii.ac.jp/crid/1070299306989168771","@type":"Researcher","foaf:name":[{"@language":"en","@value":"Wang, Sicong"}]},{"@id":"https://cir.nii.ac.jp/crid/1070299306989168640","@type":"Researcher","foaf:name":[{"@language":"en","@value":"Yang, Hui"}]},{"@id":"https://cir.nii.ac.jp/crid/1070299306989168643","@type":"Researcher","foaf:name":[{"@language":"en","@value":"Zhang, Qitao"}]},{"@id":"https://cir.nii.ac.jp/crid/1070299306989168768","@type":"Researcher","foaf:name":[{"@language":"en","@value":"Wang, 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Naoya"},{"@language":"ja","@value":"村上, 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照尚"},{"@language":"en","@value":"Ohno, Teruhisa"},{"@language":"ja-Kana","@value":"オウノ, テルヒサ"}]}],"publication":{"publicationIdentifier":[{"@type":"EISSN","@value":"18733875"},{"@type":"PISSN","@value":"0926860X"},{"@type":"NCID","@value":"AA10821202"}],"prism:publicationName":[{"@language":"en","@value":"Applied Catalysis A: General"}],"dc:publisher":[{"@value":"Elsevier"}],"prism:publicationDate":"2022-02-23","prism:volume":"634","prism:startingPage":"118539"},"reviewed":"false","url":[{"@id":"https://kyutech.repo.nii.ac.jp/records/2000374"},{"@id":"https://api.elsevier.com/content/article/PII:S0926860X2200062X?httpAccept=text/xml"},{"@id":"https://api.elsevier.com/content/article/PII:S0926860X2200062X?httpAccept=text/plain"}],"foaf:topic":[{"@id":"https://cir.nii.ac.jp/all?q=TiO2","dc:title":"TiO2"},{"@id":"https://cir.nii.ac.jp/all?q=Indoor%20VOCs%20degradation","dc:title":"Indoor VOCs degradation"},{"@id":"https://cir.nii.ac.jp/all?q=Visible%20light%20sensitizers","dc:title":"Visible light sensitizers"},{"@id":"https://cir.nii.ac.jp/all?q=Pt%20oxide%20sensitizer","dc:title":"Pt oxide sensitizer"},{"@id":"https://cir.nii.ac.jp/all?q=Fe%20oxide%20sensitizer","dc:title":"Fe oxide sensitizer"}],"dcterms:subject":[{"subjectScheme":"Other","notation":[{"@value":"TiO2"}]},{"subjectScheme":"Other","notation":[{"@value":"Indoor VOCs degradation"}]},{"subjectScheme":"Other","notation":[{"@value":"Visible light sensitizers"}]},{"subjectScheme":"Other","notation":[{"@value":"Pt oxide sensitizer"}]},{"subjectScheme":"Other","notation":[{"@value":"Fe oxide sensitizer"}]}],"project":[{"@id":"https://cir.nii.ac.jp/crid/1040003825723447936","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"20K05666"},{"@type":"JGN","@value":"JP20K05666"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-20K05666/"}],"notation":[{"@language":"ja","@value":"トラップ電子を利用した新規光触媒反応系の構築と反応機構の解明"},{"@language":"en","@value":"Development of a novel photocatalytic reaction system using photocatalytically accumulated electrons"}]},{"@id":"https://cir.nii.ac.jp/crid/1040285300695746560","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"20H02847"},{"@type":"JGN","@value":"JP20H02847"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-20H02847/"}],"notation":[{"@language":"ja","@value":"第１５属元素が配位した窒化炭素による過酸化水素生成の動作機構解明とシステム開発"},{"@language":"en","@value":"Elucidation of Reaction Mechanism and System Development of Hydrogen Peroxide Generation by Carbon Nitride Coordinated with Group 15 Element"}]},{"@id":"https://cir.nii.ac.jp/crid/1040285300696886528","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"20H05107"},{"@type":"JGN","@value":"JP20H05107"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PUBLICLY-20H05107/"}],"notation":[{"@language":"ja","@value":"光音響効果を用いた光触媒反応の「真の」量子効率測定"},{"@language":"en","@value":"Determination of the internal quantum efficiency for photocatalytic reaction over semiconductor particles by photoacoustic detection"}]}],"relatedProduct":[{"@id":"https://cir.nii.ac.jp/crid/1050010293459398400","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["references"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Trapping-Induced Enhancement of Photocatalytic Activity on Brookite TiO2 Powders: Comparison with Anatase and Rutile TiO2 Powders"},{"@value":"Trapping-Induced Enhancement of Photocatalytic Activity on Brookite TiO<sub>2</sub> Powders: Comparison with Anatase and Rutile 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light"},{"@value":"Boosting hydrogen peroxide production of brookite TiO<sub>2</sub> with Au and MXene co-catalysis under UV light"}]},{"@id":"https://cir.nii.ac.jp/crid/1360011143777367808","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Synthesis and VOC degradation ability of a CeO 2 /WO 3  thin-layer visible-light photocatalyst"}]},{"@id":"https://cir.nii.ac.jp/crid/1360011144333690368","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Investigation of multiplet splitting of Fe 2p XPS spectra and bonding in iron compounds"}]},{"@id":"https://cir.nii.ac.jp/crid/1360011146312958208","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Emission rates of indoor ozone emission devices: A literature review"}]},{"@id":"https://cir.nii.ac.jp/crid/1360013171708255616","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Ferrous iron sorption by hydrous metal 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activity of novel Pt/C-doped TiO2/PtCl4 three-component nanojunction system for degradation of toluene in air"}]},{"@id":"https://cir.nii.ac.jp/crid/1360013172907565440","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Influences of pH value in deposition-precipitation synthesis process on Pt-doped TiO2 catalysts for photocatalytic oxidation of NO"}]},{"@id":"https://cir.nii.ac.jp/crid/1360013173075761024","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Key role of local acetaldehyde in upper GI tract carcinogenesis"}]},{"@id":"https://cir.nii.ac.jp/crid/1360013200109642112","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Discussion on the health problems of indoor living"}]},{"@id":"https://cir.nii.ac.jp/crid/1360017280643593984","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Enhanced photocatalytic VOCs 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processes"}]},{"@id":"https://cir.nii.ac.jp/crid/1360294647030697856","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Improved C-history method for rapidly and accurately measuring the characteristic parameters of formaldehyde/VOCs emitted from building materials"}]},{"@id":"https://cir.nii.ac.jp/crid/1360294647469749376","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Pt Nanoparticle-Decorated CdS Photocalysts for CO<sub>2</sub> Reduction and H<sub>2</sub> Evolution"}]},{"@id":"https://cir.nii.ac.jp/crid/1360294648071856512","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Adsorption and Photocatalytic Kinetics of Visible-Light Response N-Doped TiO<sub>2</sub>Nanocatalyst for Indoor Acetaldehyde Removal under Dark and Light Conditions"}]},{"@id":"https://cir.nii.ac.jp/crid/1360574094716547712","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Highly 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