{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1050865950561860864.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"HDL","@value":"https://hdl.handle.net/2324/7162498"}},{"identifier":{"@type":"DOI","@value":"10.1002/adfm.202312645"}},{"identifier":{"@type":"URI","@value":"https://advanced.onlinelibrary.wiley.com/doi/pdf/10.1002/adfm.202312645"}}],"resourceType":"学術雑誌論文(journal article)","dc:title":[{"@language":"en","@value":"Realizing Super-High Piezoelectricity and Excellent Fatigue Resistance in Domain-Engineered Bismuth Titanate Ferroelectrics"},{"@value":"Realizing Super‐High Piezoelectricity and Excellent Fatigue Resistance in Domain‐Engineered Bismuth Titanate Ferroelectrics"}],"dc:language":"en","description":[{"type":"Abstract","notation":[{"@language":"en","@value":"Bismuth titanate (BIT) is widely known as one of the most prospective lead-free ferroelectric and piezoelectric materials in advanced high-temperature sensing applications. Despite significant advances in developing BIT ferroelectrics, it still faces major scientific and engineering challenges in realizing super-high performance to meet next-generation high-sensitivity and light-weight applications. Here, a novel ferroelectric domain-engineered BIT ceramic system is conceived that exhibits super-high piezoelectric coefficient (d33 = 38.5 pC N−1) and inverse piezoelectric coefficient (d33* = 46.7 pm V−1) at low electric field as well as excellent fatigue resistance (stable up to 107 cycles). The results reveal that the introduction of high-density layered (001)-type 180° domain walls with flexible polarization rotation features and the formation of small-size multi-domain states with low energy barriers are mainly responsible for the excellent electrical performance. To the best of knowledge, it is the first time to reveal such intriguing domain structures in BIT ceramics in detail, especially from the atomic-scale perspective by using atomic number (Z)-contrast imaging in combination with atomic-resolution polarization mapping. It is believed that this breakthrough conduces to comprehensively understand structural features of ferroelectric domains in BIT ceramics, and also opens a window for future developments of super-high performance in bismuth layer-structured ferroelectrics via domain engineering."}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1030015487558574464","@type":"Researcher","personIdentifier":[{"@type":"ORCID","@value":"0000-0002-8173-2507"}],"foaf:name":[{"@language":"en","@value":"Xie, Shaoxiong"}],"jpcoar:affiliationName":[{"@language":"en","@value":"Institute for Advanced Study, Chengdu University"},{"@language":"en","@value":"Department of Mechanical Engineering, Kyushu University"},{"@language":"ja","@value":"九州大学大学院工学研究院機械工学部門"}]},{"@id":"https://cir.nii.ac.jp/crid/1070865950561860868","@type":"Researcher","foaf:name":[{"@language":"en","@value":"Xu, Qian"}],"jpcoar:affiliationName":[{"@language":"en","@value":"School of Architecture and Civil Engineering, Xihua University"}]},{"@id":"https://cir.nii.ac.jp/crid/1420845751138234368","@type":"Researcher","personIdentifier":[{"@type":"KAKEN_RESEARCHERS","@value":"30264451"},{"@type":"NRID","@value":"1000030264451"},{"@type":"NRID","@value":"9000020832549"},{"@type":"NRID","@value":"9000021281467"},{"@type":"NRID","@value":"9000021283149"},{"@type":"NRID","@value":"9000003724147"},{"@type":"NRID","@value":"9000309165948"},{"@type":"RESEARCHMAP","@value":"https://researchmap.jp/_John"}],"foaf:name":[{"@language":"en","@value":"Chen, Qiang"},{"@language":"ja","@value":"陳, 強"},{"@language":"ja-Kana","@value":"ツエン, チアン"}],"jpcoar:affiliationName":[{"@language":"en","@value":"Department of Mechanical Engineering, Kyushu University"},{"@language":"ja","@value":"九州大学大学院工学研究院機械工学部門"}]},{"@id":"https://cir.nii.ac.jp/crid/1070865950561860867","@type":"Researcher","foaf:name":[{"@language":"en","@value":"Zhu, Jianguo"}],"jpcoar:affiliationName":[{"@language":"en","@value":"College of Materials Science and Engineering, Sichuan University"}]},{"@id":"https://cir.nii.ac.jp/crid/1070865950561860866","@type":"Researcher","foaf:name":[{"@language":"en","@value":"Wang, Qingyuan"}],"jpcoar:affiliationName":[{"@language":"en","@value":"Institute for Advanced Study, Chengdu University"}]}],"publication":{"publicationIdentifier":[{"@type":"PISSN","@value":"1616301X"},{"@type":"EISSN","@value":"16163028"},{"@type":"NCID","@value":"AA11518753"}],"prism:publicationName":[{"@language":"en","@value":"Advanced Functional Materials"}],"dc:publisher":[{"@value":"Wiley"}],"prism:publicationDate":"2024-01-20","prism:volume":"34","prism:number":"18","prism:startingPage":"2312645"},"reviewed":"false","dcterms:accessRights":"http://purl.org/coar/access_right/c_abf2","url":[{"@id":"https://advanced.onlinelibrary.wiley.com/doi/pdf/10.1002/adfm.202312645"}],"foaf:topic":[{"@id":"https://cir.nii.ac.jp/all?q=Bismuth%20titanate","dc:title":"Bismuth titanate"},{"@id":"https://cir.nii.ac.jp/all?q=Electrical%20performance","dc:title":"Electrical performance"},{"@id":"https://cir.nii.ac.jp/all?q=Lattice%20distortion","dc:title":"Lattice distortion"},{"@id":"https://cir.nii.ac.jp/all?q=Domain%20structures","dc:title":"Domain structures"},{"@id":"https://cir.nii.ac.jp/all?q=Atomic%20resolution%20polarization%20mapping","dc:title":"Atomic resolution polarization mapping"}],"dcterms:subject":[{"subjectScheme":"Other","notation":[{"@language":"en","@value":"Bismuth titanate"}]},{"subjectScheme":"Other","notation":[{"@language":"en","@value":"Electrical performance"}]},{"subjectScheme":"Other","notation":[{"@language":"en","@value":"Lattice distortion"}]},{"subjectScheme":"Other","notation":[{"@language":"en","@value":"Domain structures"}]},{"subjectScheme":"Other","notation":[{"@language":"en","@value":"Atomic resolution polarization mapping"}]}],"project":[{"@id":"https://cir.nii.ac.jp/crid/1040010457589142144","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"22K03828"},{"@type":"JGN","@value":"JP22K03828"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-22K03828/"}],"notation":[{"@language":"ja","@value":"精密構造解析による階層異方性ナノ構造合金の超高サイクル疲労強度発見機構の解明"},{"@language":"en","@value":"Ultra-high cycle fatigue strength of hierarchical anisotropic nanostructured alloys by precision structural analysis"}]},{"@id":"https://cir.nii.ac.jp/crid/1040577354307811840","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"22KF0290"},{"@type":"JGN","@value":"JP22KF0290"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-22KF0290/"}],"notation":[{"@language":"ja","@value":"チタン酸ビスマス高温圧電セラミックのドメイン構造と分極ダイナミクス"},{"@language":"en","@value":"Bismuth titanate-based high temperature piezoceramics: Domain structure and polarization 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