{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1360004229884041344.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1002/advs.201800384"}},{"identifier":{"@type":"URI","@value":"https://api.wiley.com/onlinelibrary/tdm/v1/articles/10.1002%2Fadvs.201800384"}},{"identifier":{"@type":"URI","@value":"https://advanced.onlinelibrary.wiley.com/doi/pdf/10.1002/advs.201800384"}},{"identifier":{"@type":"PMID","@value":"29938193"}}],"resourceType":"学術雑誌論文(journal article)","dc:title":[{"@value":"A Nacre‐Like Carbon Nanotube Sheet for High Performance Li‐Polysulfide Batteries with High Sulfur Loading"}],"description":[{"type":"abstract","notation":[{"@value":"<jats:title>Abstract</jats:title><jats:p>Lithium‐sulfur (Li‐S) batteries are considered as one of the most promising energy storage systems for next‐generation electric vehicles because of their high‐energy density. However, the poor cyclic stability, especially at a high sulfur loading, is the major obstacles retarding their practical use. Inspired by the nacre structure of an abalone, a similar configuration consisting of layered carbon nanotube (CNT) matrix and compactly embedded sulfur is designed as the cathode for Li‐S batteries, which are realized by a well‐designed unidirectional freeze‐drying approach. The compact and lamellar configuration with closely contacted neighboring CNT layers and the strong interaction between the highly conductive network and polysulfides have realized a high sulfur loading with significantly restrained polysulfide shuttling, resulting in a superior cyclic stability and an excellent rate performance for the produced Li‐S batteries. Typically, with a sulfur loading of 5 mg cm<jats:sup>−2</jats:sup>, the assembled batteries demonstrate discharge capacities of 1236 mAh g<jats:sup>−1</jats:sup> at 0.1 C, 498 mAh g<jats:sup>−1</jats:sup> at 2 C and moreover, when the sulfur loading is further increased to 10 mg cm<jats:sup>−2</jats:sup> coupling with a carbon‐coated separator, a superhigh areal capacity of 11.0 mAh cm<jats:sup>−2</jats:sup> is achieved.</jats:p>"}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1380298336739069440","@type":"Researcher","foaf:name":[{"@value":"Zheng‐Ze Pan"}],"jpcoar:affiliationName":[{"@value":"Engineering Laboratory for Functionalized Carbon Materials Shenzhen Key Laboratory for Graphene‐based Materials Graduate School at Shenzhen Tsinghua University  Shenzhen 518055 China"},{"@value":"School of Materials Science and Engineering Tsinghua University  Beijing 100084 China"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229884041483","@type":"Researcher","foaf:name":[{"@value":"Wei Lv"}],"jpcoar:affiliationName":[{"@value":"Engineering Laboratory for Functionalized Carbon Materials Shenzhen Key Laboratory for Graphene‐based Materials Graduate School at Shenzhen Tsinghua University  Shenzhen 518055 China"}]},{"@id":"https://cir.nii.ac.jp/crid/1380298336739069441","@type":"Researcher","foaf:name":[{"@value":"Yan‐Bing He"}],"jpcoar:affiliationName":[{"@value":"Engineering Laboratory for Functionalized Carbon Materials Shenzhen Key Laboratory for Graphene‐based Materials Graduate School at Shenzhen Tsinghua University  Shenzhen 518055 China"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229884041349","@type":"Researcher","foaf:name":[{"@value":"Yan Zhao"}],"jpcoar:affiliationName":[{"@value":"Engineering Laboratory for Functionalized Carbon Materials Shenzhen Key Laboratory for Graphene‐based Materials Graduate School at Shenzhen Tsinghua University  Shenzhen 518055 China"},{"@value":"School of Materials Science and Engineering Tsinghua University  Beijing 100084 China"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229884041476","@type":"Researcher","foaf:name":[{"@value":"Guangmin Zhou"}],"jpcoar:affiliationName":[{"@value":"Department of Materials Science and Engineering Stanford University  Stanford CA 94305 USA"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229884041617","@type":"Researcher","foaf:name":[{"@value":"Liubing Dong"}],"jpcoar:affiliationName":[{"@value":"Engineering Laboratory for Functionalized Carbon Materials Shenzhen Key Laboratory for Graphene‐based Materials Graduate School at Shenzhen Tsinghua University  Shenzhen 518055 China"},{"@value":"School of Materials Science and Engineering Tsinghua University  Beijing 100084 China"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229884041728","@type":"Researcher","foaf:name":[{"@value":"Shuzhang Niu"}],"jpcoar:affiliationName":[{"@value":"Tsinghua‐Berkeley Shenzhen Institute (TBSI) Tsinghua University  Shenzhen 518055 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Beijing 100084 China"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229884041486","@type":"Researcher","foaf:name":[{"@value":"Huifa Shi"}],"jpcoar:affiliationName":[{"@value":"Engineering Laboratory for Functionalized Carbon Materials Shenzhen Key Laboratory for Graphene‐based Materials Graduate School at Shenzhen Tsinghua University  Shenzhen 518055 China"},{"@value":"School of Materials Science and Engineering Tsinghua University  Beijing 100084 China"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229884041357","@type":"Researcher","foaf:name":[{"@value":"Wenjie Zhang"}],"jpcoar:affiliationName":[{"@value":"School of Materials Science and Engineering Tsinghua University  Beijing 100084 China"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229884041611","@type":"Researcher","foaf:name":[{"@value":"Feiyu Kang"}],"jpcoar:affiliationName":[{"@value":"Engineering Laboratory for Functionalized Carbon Materials Shenzhen Key Laboratory for Graphene‐based Materials Graduate School at Shenzhen Tsinghua University  Shenzhen 518055 China"},{"@value":"School of Materials Science and Engineering Tsinghua University  Beijing 100084 China"},{"@value":"Tsinghua‐Berkeley Shenzhen Institute (TBSI) Tsinghua University  Shenzhen 518055 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Nishihara"}],"jpcoar:affiliationName":[{"@value":"Institute of Multidisciplinary Research for Advanced Materials Tohoku University  Sendai 980−8577 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380298336739069312","@type":"Researcher","foaf:name":[{"@value":"Quan‐Hong Yang"}],"jpcoar:affiliationName":[{"@value":"Engineering Laboratory for Functionalized Carbon Materials Shenzhen Key Laboratory for Graphene‐based Materials Graduate School at Shenzhen Tsinghua University  Shenzhen 518055 China"},{"@value":"Tsinghua‐Berkeley Shenzhen Institute (TBSI) Tsinghua University  Shenzhen 518055 China"},{"@value":"School of Chemical Engineering and Technology Tianjin University  Tianjin 300072 China"}]}],"publication":{"publicationIdentifier":[{"@type":"PISSN","@value":"21983844"},{"@type":"EISSN","@value":"21983844"}],"prism:publicationName":[{"@value":"Advanced Science"}],"dc:publisher":[{"@value":"Wiley"}],"prism:publicationDate":"2018-04-19","prism:volume":"5","prism:number":"6","prism:startingPage":"1800384"},"reviewed":"false","dcterms:accessRights":"http://purl.org/coar/access_right/c_abf2","dc:rights":["http://creativecommons.org/licenses/by/4.0/"],"url":[{"@id":"https://api.wiley.com/onlinelibrary/tdm/v1/articles/10.1002%2Fadvs.201800384"},{"@id":"https://advanced.onlinelibrary.wiley.com/doi/pdf/10.1002/advs.201800384"}],"createdAt":"2018-04-19","modifiedAt":"2025-10-06","foaf:topic":[{"@id":"https://cir.nii.ac.jp/all?q=high%20sulfur%20loading","dc:title":"high sulfur loading"},{"@id":"https://cir.nii.ac.jp/all?q=Science","dc:title":"Science"},{"@id":"https://cir.nii.ac.jp/all?q=carbon%20nanotube%20sheets","dc:title":"carbon nanotube sheets"},{"@id":"https://cir.nii.ac.jp/all?q=Q","dc:title":"Q"},{"@id":"https://cir.nii.ac.jp/all?q=nacre%E2%80%90like%20materials","dc:title":"nacre‐like materials"},{"@id":"https://cir.nii.ac.jp/all?q=Li%E2%80%90polysulfide%20batteries","dc:title":"Li‐polysulfide batteries"},{"@id":"https://cir.nii.ac.jp/all?q=Communications","dc:title":"Communications"},{"@id":"https://cir.nii.ac.jp/all?q=Li%E2%80%90sulfur%20batteries","dc:title":"Li‐sulfur batteries"}],"project":[{"@id":"https://cir.nii.ac.jp/crid/1040000781954055424","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"17H01042"},{"@type":"JGN","@value":"JP17H01042"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-17H01042/"}],"notation":[{"@language":"ja","@value":"単層グラフェン多孔体の展開研究"},{"@language":"en","@value":"Development of porous materials with single-graphene walls"}]}],"relatedProduct":[{"@id":"https://cir.nii.ac.jp/crid/1360004230302745600","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"A Directional Strain Sensor Based on Anisotropic Microhoneycomb Cellulose 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