{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1360004229922752128.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1002/anie.201510000"}},{"identifier":{"@type":"URI","@value":"https://api.wiley.com/onlinelibrary/tdm/v1/articles/10.1002%2Fanie.201510000"}},{"identifier":{"@type":"URI","@value":"https://onlinelibrary.wiley.com/doi/pdf/10.1002/anie.201510000"}},{"identifier":{"@type":"DOI","@value":"10.1002/ange.201510000"}},{"identifier":{"@type":"PMID","@value":"26891152"}}],"resourceType":"学術雑誌論文(journal article)","dc:title":[{"@value":"Remarkable Charge Separation and Photocatalytic Efficiency Enhancement through Interconnection of TiO<sub>2</sub> Nanoparticles by Hydrothermal Treatment"}],"description":[{"type":"abstract","notation":[{"@value":"<jats:title>Abstract</jats:title><jats:p>Although tremendous effort has been directed to synthesizing advanced TiO<jats:sub>2</jats:sub>, it remains difficult to obtain TiO<jats:sub>2</jats:sub> exhibiting a photocatalytic efficiency higher than that of P25, a benchmark photocatalyst. P25 is composed of anatase, rutile, and amorphous TiO<jats:sub>2</jats:sub> particles, and photoexcited electron transfer and subsequent charge separation at the anatase–rutile particle interfaces explain its high photocatalytic efficiency. Herein, we report on a facile and rational hydrothermal treatment of P25 to selectively convert the amorphous component into crystalline TiO<jats:sub>2</jats:sub>, which is deposited between the original anatase and rutile particles to increase the particle interfaces and thus enhance charge separation. This process produces a new TiO<jats:sub>2</jats:sub> exhibiting a considerably enhanced photocatalytic efficiency. This method of synthesizing this TiO<jats:sub>2</jats:sub>, inspired by a recently burgeoning zeolite design, promises to make TiO<jats:sub>2</jats:sub> applications more feasible and effective.</jats:p>"}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1420282801197324544","@type":"Researcher","personIdentifier":[{"@type":"KAKEN_RESEARCHERS","@value":"40449327"},{"@type":"NRID","@value":"1000040449327"},{"@type":"NRID","@value":"9000412605233"},{"@type":"NRID","@value":"9000370746442"},{"@type":"NRID","@value":"9000325953937"}],"foaf:name":[{"@value":"Yusuke Ide"}],"jpcoar:affiliationName":[{"@value":"International Center for Materials Nanoarchitectonics (MANA) National Institute for Materials Science (NIMS)  1-1 Namiki, Tsukuba Ibaraki 305-0044 Japan"},{"@value":"Graduate School of Creative Science and Engineering Waseda University  1-6-1 Nishiwaseda, Shinjuku-ku Tokyo 169–8050 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229922752004","@type":"Researcher","foaf:name":[{"@value":"Nozomu Inami"}],"jpcoar:affiliationName":[{"@value":"Department of Earth Sciences Waseda University  1-6-1 Nishiwaseda, Shinjuku-ku Tokyo 169–8050 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229922752009","@type":"Researcher","foaf:name":[{"@value":"Hideya Hattori"}],"jpcoar:affiliationName":[{"@value":"Graduate School of Engineering Department of Applied Chemistry Hiroshima University  1-4-1 Kagamiyama Higashi-Hiroshima 739-8527 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229922752007","@type":"Researcher","foaf:name":[{"@value":"Kanji Saito"}],"jpcoar:affiliationName":[{"@value":"Department of Earth Sciences Waseda University  1-6-1 Nishiwaseda, Shinjuku-ku Tokyo 169–8050 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229922752017","@type":"Researcher","foaf:name":[{"@value":"Minoru Sohmiya"}],"jpcoar:affiliationName":[{"@value":"Department of Earth Sciences Waseda University  1-6-1 Nishiwaseda, Shinjuku-ku Tokyo 169–8050 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229922752135","@type":"Researcher","foaf:name":[{"@value":"Nao Tsunoji"}],"jpcoar:affiliationName":[{"@value":"Graduate School of Engineering Department of Applied Chemistry Hiroshima University  1-4-1 Kagamiyama Higashi-Hiroshima 739-8527 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229922752014","@type":"Researcher","foaf:name":[{"@value":"Kenji Komaguchi"}],"jpcoar:affiliationName":[{"@value":"Graduate School of Engineering Department of Applied Chemistry Hiroshima University  1-4-1 Kagamiyama Higashi-Hiroshima 739-8527 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229922752136","@type":"Researcher","foaf:name":[{"@value":"Tsuneji Sano"}],"jpcoar:affiliationName":[{"@value":"Graduate School of Engineering Department of Applied Chemistry Hiroshima University  1-4-1 Kagamiyama Higashi-Hiroshima 739-8527 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229922752013","@type":"Researcher","foaf:name":[{"@value":"Yoshio Bando"}],"jpcoar:affiliationName":[{"@value":"International Center for Materials Nanoarchitectonics (MANA) National Institute for Materials Science (NIMS)  1-1 Namiki, Tsukuba Ibaraki 305-0044 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229922752137","@type":"Researcher","foaf:name":[{"@value":"Dmitri Golberg"}],"jpcoar:affiliationName":[{"@value":"International Center for Materials Nanoarchitectonics (MANA) National Institute for Materials Science (NIMS)  1-1 Namiki, Tsukuba Ibaraki 305-0044 Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004229922752015","@type":"Researcher","foaf:name":[{"@value":"Yoshiyuki Sugahara"}],"jpcoar:affiliationName":[{"@value":"Graduate School of Creative Science and Engineering Waseda University  1-6-1 Nishiwaseda, Shinjuku-ku Tokyo 169–8050 Japan"},{"@value":"Department of Applied Chemistry School of Advanced Science and Engineering Waseda University  3-4-1 Ohkubo, Shinjuku-ku Tokyo 169-8555 Japan"},{"@value":"Kagami Memorial Research Institute for Materials Science and Technology Waseda University  2-8-26 Nishiwaseda, Shinjuku-ku Tokyo 169-0051 Japan"}]}],"publication":{"publicationIdentifier":[{"@type":"PISSN","@value":"14337851"},{"@type":"EISSN","@value":"15213773"}],"prism:publicationName":[{"@value":"Angewandte Chemie International Edition"}],"dc:publisher":[{"@value":"Wiley"}],"prism:publicationDate":"2016-02-17","prism:volume":"55","prism:number":"11","prism:startingPage":"3600","prism:endingPage":"3605"},"reviewed":"false","dc:rights":["http://onlinelibrary.wiley.com/termsAndConditions#vor"],"url":[{"@id":"https://api.wiley.com/onlinelibrary/tdm/v1/articles/10.1002%2Fanie.201510000"},{"@id":"https://onlinelibrary.wiley.com/doi/pdf/10.1002/anie.201510000"}],"createdAt":"2016-02-18","modifiedAt":"2023-10-06","foaf:topic":[{"@id":"https://cir.nii.ac.jp/all?q=titanium%20dioxide","dc:title":"titanium dioxide"},{"@id":"https://cir.nii.ac.jp/all?q=charge%20separation","dc:title":"charge separation"},{"@id":"https://cir.nii.ac.jp/all?q=dye-sensitized%20solar%20cell","dc:title":"dye-sensitized solar 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