{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1360004233178035584.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1021/cg501560z"}},{"identifier":{"@type":"URI","@value":"https://pubs.acs.org/doi/pdf/10.1021/cg501560z"}}],"resourceType":"学術雑誌論文(journal article)","dc:title":[{"@value":"Three-Dimensional Architectures of [Mn<sup>II</sup>Cr<sup>III</sup>(oxalate)<sub>3</sub>]<sup>−</sup> Complexes with Cage-Type Networks Surrounding Supramolecular Cations"}],"description":[{"notation":[{"@value":"Metal–organic network structure based on oxalate bridges {[MnIICrIII(oxalate)3]−}∞ and supramolecular cations (H2PPD2+)(benzo[18]crown-6)2[MnCr(oxalate)3](CH3OH)(CH3CN)2 (1) and (o-FAni+)2(DCH[18]crown-6)2[Mn(CH3OH)Cr(oxalate)3][MnCr(oxalate)3](CH3OH) (2), where H2PPD2+, o-FAni+, and DCH[18]crown-6 denote p-phenylenediammonium2+, o-fluoroanilinium+, and cis-syn-cis-dicyclohexano[18]crown-6, respectively, were synthesized. The crystal structure of 1 was the combination of [Mn(Λ)Cr(Λ)(oxalate)3]− and [Mn(Λ)Cr(Δ)(oxalate)3]−, whereas that of crystal 2 was the combination of [Mn(Λ)(CH3OH)Cr(Δ)(oxalate)3] and [Mn(Λ)Cr(Δ)(oxalate)3]. Large flexible supramolecular cations provide the three-dimensional structure of {[MnIICrIII(oxalate)3]−}∞, which is different from the two-dimensional honeycomb structure often observed for {[MnIICrIII(oxalate)3]−}∞ complexes. Temperature-dependent magnetic susceptibilities of the complexes 1 and 2 exhibited ferromagnetic behaviors following the Curie–Weiss law (C = 11.5 cm3 K mol..."}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1380004233178035584","@type":"Researcher","foaf:name":[{"@value":"Toru Endo"}],"jpcoar:affiliationName":[{"@value":"Graduate\rSchool of Environmental Science, Hokkaido University, N10W5, Kita-ku, Sapporo, 060-0810, Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004233178035588","@type":"Researcher","foaf:name":[{"@value":"Kazuya Kubo"}],"jpcoar:affiliationName":[{"@value":"Graduate\rSchool of Environmental Science, Hokkaido University, N10W5, Kita-ku, Sapporo, 060-0810, Japan"},{"@value":"Research\rInstitute for Electronic Science, Hokkaido University, N20W10, Kita-ku, Sapporo, 001-0020, Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004233178035586","@type":"Researcher","foaf:name":[{"@value":"Masashi Yoshitake"}],"jpcoar:affiliationName":[{"@value":"Research\rInstitute for 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Nakamura"}],"jpcoar:affiliationName":[{"@value":"Graduate\rSchool of Environmental Science, Hokkaido University, N10W5, Kita-ku, Sapporo, 060-0810, Japan"},{"@value":"Research\rInstitute for Electronic Science, Hokkaido University, N20W10, Kita-ku, Sapporo, 001-0020, Japan"}]}],"publication":{"publicationIdentifier":[{"@type":"PISSN","@value":"15287483"},{"@type":"EISSN","@value":"15287505"}],"prism:publicationName":[{"@value":"Crystal Growth & Design"}],"dc:publisher":[{"@value":"American Chemical Society (ACS)"}],"prism:publicationDate":"2015-02-05","prism:volume":"15","prism:number":"3","prism:startingPage":"1186","prism:endingPage":"1193"},"reviewed":"false","dcterms:accessRights":"http://purl.org/coar/access_right/c_abf2","invited":"false","url":[{"@id":"https://pubs.acs.org/doi/pdf/10.1021/cg501560z"}],"createdAt":"2015-01-21","modifiedAt":"2023-04-18","project":[{"@id":"https://cir.nii.ac.jp/crid/1040000782144603648","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"23245027"},{"@type":"JGN","@value":"JP23245027"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-23245027/"}],"notation":[{"@language":"ja","@value":"分子回転とマクロ物性の融合"},{"@language":"en","@value":"Molecular Rotation and Macofunctions"}]},{"@id":"https://cir.nii.ac.jp/crid/1040000782298135040","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"26410064"},{"@type":"JGN","@value":"JP26410064"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-26410064/"}],"notation":[{"@language":"ja","@value":"超分子ローターによる金属錯体の相転移制御"},{"@language":"en","@value":"Tuning phase transitions of bistable metal complexes with supramolecular rotators"}]},{"@id":"https://cir.nii.ac.jp/crid/1040282256806163712","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"15H03791"},{"@type":"JGN","@value":"JP15H03791"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-15H03791/"}],"notation":[{"@language":"ja","@value":"分子性スーパープロトンリレー材料の創製"},{"@language":"en","@value":"Fabrication of Molecular Super Proton Relay Material"}]},{"@id":"https://cir.nii.ac.jp/crid/1040282257185229696","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"24550068"},{"@type":"JGN","@value":"JP24550068"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-24550068/"}],"notation":[{"@language":"ja","@value":"電荷分離型中性配位子を利用した多孔性軽金属錯体の構造多様化"},{"@language":"en","@value":"Structural diversification of porous light metal complexes using charge-separated neutral 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