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The formation of bPEB in the excited singlet state ((1)bPEB*) can be attributed to the charge recombination between bPEB(*+) and bPEB(*-), which are initially generated from the radiolytic reaction. This mechanism is reasonably explained by the relationship between the annihilation enthalpy change (-DeltaH(o)) for the charge recombination of bPEB(*+) and bPEB(*-) and excitation energy of (1)bPEB*. Since the degree of the pi-conjugation in the S(1) state and HOMO-LUMO levels of bPEB change with the substitution pattern of phenylacetylene groups on the central benzene ring and the various kinds of donor and/or acceptor group, the fine-tuning of the emission color and intensity of bPEB can be easily carried out during pulse radiolysis in Bz. For donor-acceptor-substituted bPEB, it was found that the difference in the charge transfer conjugated pathways between donor and acceptor substituents (linear-, cross-, and \"bent\"-conjugated pathways) strongly influenced the HOMO-LUMO energy gap."}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1380004233230366338","@type":"Researcher","foaf:name":[{"@value":"Shingo Samori"}],"jpcoar:affiliationName":[{"@value":"The Institute of Scientific and Industrial Research (SANKEN), Osaka University, Mihogaoka 8-1, Ibaraki, Osaka 567-0047, Japan, and Department of Chemistry and the Materials Science Institute, University of Oregon, Eugene, Oregon 97403-1253"}]},{"@id":"https://cir.nii.ac.jp/crid/1420001326221271296","@type":"Researcher","personIdentifier":[{"@type":"KAKEN_RESEARCHERS","@value":"50197844"},{"@type":"NRID","@value":"1000050197844"},{"@type":"NRID","@value":"9000001729094"},{"@type":"NRID","@value":"9000257715360"},{"@type":"NRID","@value":"9000238422252"},{"@type":"NRID","@value":"9000258602070"},{"@type":"NRID","@value":"9000000659904"},{"@type":"NRID","@value":"9000000462919"},{"@type":"NRID","@value":"9000378106252"},{"@type":"NRID","@value":"9000345257249"},{"@type":"NRID","@value":"9000256025150"},{"@type":"NRID","@value":"9000258594237"},{"@type":"NRID","@value":"9000255702929"},{"@type":"NRID","@value":"9000329004012"},{"@type":"RESEARCHMAP","@value":"https://researchmap.jp/read0014188"}],"foaf:name":[{"@value":"Sachiko Tojo"}],"jpcoar:affiliationName":[{"@value":"The Institute of Scientific and Industrial Research (SANKEN), Osaka University, Mihogaoka 8-1, Ibaraki, Osaka 567-0047, Japan, and Department of Chemistry and the Materials Science Institute, University of Oregon, Eugene, Oregon 97403-1253"}]},{"@id":"https://cir.nii.ac.jp/crid/1420001326231446656","@type":"Researcher","personIdentifier":[{"@type":"KAKEN_RESEARCHERS","@value":"40282040"},{"@type":"NRID","@value":"1000040282040"},{"@type":"NRID","@value":"9000005680778"},{"@type":"NRID","@value":"9000001729095"},{"@type":"NRID","@value":"9000298976634"},{"@type":"NRID","@value":"9000020626793"},{"@type":"NRID","@value":"9000255700374"},{"@type":"NRID","@value":"9000257717373"},{"@type":"NRID","@value":"9000015544886"},{"@type":"NRID","@value":"9000256029846"},{"@type":"NRID","@value":"9000256020060"},{"@type":"NRID","@value":"9000257715085"},{"@type":"NRID","@value":"9000257718268"},{"@type":"NRID","@value":"9000390918531"},{"@type":"NRID","@value":"9000000827364"},{"@type":"NRID","@value":"9000255701021"},{"@type":"NRID","@value":"9000258594273"},{"@type":"NRID","@value":"9000257716856"},{"@type":"NRID","@value":"9000412104479"},{"@type":"NRID","@value":"9000383699739"},{"@type":"NRID","@value":"9000283740697"},{"@type":"NRID","@value":"9000257716267"},{"@type":"NRID","@value":"9000378106255"},{"@type":"NRID","@value":"9000345257250"},{"@type":"NRID","@value":"9000001219995"},{"@type":"NRID","@value":"9000257713923"},{"@type":"NRID","@value":"9000409600086"},{"@type":"NRID","@value":"9000255701779"},{"@type":"NRID","@value":"9000256023784"},{"@type":"NRID","@value":"9000401668809"},{"@type":"NRID","@value":"9000255700740"},{"@type":"NRID","@value":"9000415350196"},{"@type":"NRID","@value":"9000001219684"},{"@type":"NRID","@value":"9000255702928"},{"@type":"NRID","@value":"9000256017461"},{"@type":"NRID","@value":"9000329004013"},{"@type":"NRID","@value":"9000399166412"},{"@type":"NRID","@value":"9000255700131"},{"@type":"NRID","@value":"9000256022857"},{"@type":"NRID","@value":"9000258595745"},{"@type":"NRID","@value":"9000257708810"},{"@type":"RESEARCHMAP","@value":"https://researchmap.jp/read0118564"}],"foaf:name":[{"@value":"Mamoru Fujitsuka"}],"jpcoar:affiliationName":[{"@value":"The Institute of Scientific and Industrial Research (SANKEN), Osaka University, Mihogaoka 8-1, Ibaraki, Osaka 567-0047, Japan, and Department of Chemistry and the Materials Science Institute, University of Oregon, Eugene, Oregon 97403-1253"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004233230366340","@type":"Researcher","foaf:name":[{"@value":"Torben Ryhding"}],"jpcoar:affiliationName":[{"@value":"The Institute of Scientific and Industrial Research (SANKEN), Osaka University, Mihogaoka 8-1, Ibaraki, Osaka 567-0047, Japan, and Department of Chemistry and the Materials Science Institute, University of Oregon, Eugene, Oregon 97403-1253"}]},{"@id":"https://cir.nii.ac.jp/crid/1380004233230366339","@type":"Researcher","foaf:name":[{"@value":"Aaron G. 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