{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1360021390742914560.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1021/acsaelm.3c00845"}},{"identifier":{"@type":"URI","@value":"https://pubs.acs.org/doi/pdf/10.1021/acsaelm.3c00845"}}],"resourceType":"学術雑誌論文(journal article)","dc:title":[{"@value":"Supramolecular Self-Assembly of Diketopyrrolopyrrole with Unprecedented Photoconductivity"}],"description":[{"notation":[{"@value":"The oscillation of chemical bonds in molecular semiconductors plays a key role in fragmenting the electric conducting pathways due to the large fraction of free volumes, acting as “trap sites” for charge carriers. Incorporating directional noncovalent chemical bonds between the monomeric unit in organic semiconductors is an excellent approach to reducing thermally induced structural fluctuations, resulting in a decrease in a trap densities. In this work, we utilize noncovalent interactions in diketopyrrolopyrrole (DPP)-based supramolecular assembled systems to enhance or tune the photoconductivity and charge transport properties. Infinitesimal molecular design by substituting different side chains and introducing intramolecular dihedral angles leads to a notable difference in solid-state packing, transient photoconductivity, and thin film morphology. Grazing incidence wide-angle X-ray scattering, and thin film X-ray diffraction measurements reveal that the packing order is enhanced for hexyl substituted DPP derivatives, resulting in high intrinsic charge carrier mobility of $∑μ$ = 1.7 cm$^2$ V$^{–1}$ s$^{–1}$. At the microscopic level, electron microscopy reveals that the unique self-assembly remarkably improves the structural order via directional hydrogen bonding. These findings exemplify that the supramolecular self-assembly strategy via hydrogen bonding networks is an efficacious way to reduce the molecular vibration and structural defects in molecular semiconductors and ameliorate the performance in optoelectronic devices."}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1380021390742914564","@type":"Researcher","foaf:name":[{"@value":"Nilabja Maity"}],"jpcoar:affiliationName":[{"@value":"Solid State and Structural Chemistry Unit, Indian Institute of Science, Bangalore 560012, India"}]},{"@id":"https://cir.nii.ac.jp/crid/1380021390742914563","@type":"Researcher","foaf:name":[{"@value":"Manoj Kumar Sharma"}],"jpcoar:affiliationName":[{"@value":"Solid State and Structural Chemistry Unit, Indian Institute of Science, Bangalore 560012, India"}]},{"@id":"https://cir.nii.ac.jp/crid/1380021390742914567","@type":"Researcher","foaf:name":[{"@value":"Samrat Ghosh"}],"jpcoar:affiliationName":[{"@value":"Department of Molecular Engineering, Kyoto University, Nishikyo-ku, Kyoto 615-8510, Japan"},{"@value":"Inorganic and Physical Chemistry Laboratory, CSIR−Central Leather Research Institute, Chennai 600020, India"}]},{"@id":"https://cir.nii.ac.jp/crid/1380021390742914560","@type":"Researcher","foaf:name":[{"@value":"Mathias K. Huss-Hansen"}],"jpcoar:affiliationName":[{"@value":"NanoSYD, Mads Clausen Institute, University of Southern Denmark, 6400 Sønderborg, Denmark"}]},{"@id":"https://cir.nii.ac.jp/crid/1380021390742914688","@type":"Researcher","foaf:name":[{"@value":"Ahin Roy"}],"jpcoar:affiliationName":[{"@value":"Materials Research Centre, Indian Institute of Science, Bangalore 560012, India"}]},{"@id":"https://cir.nii.ac.jp/crid/1380021390742914565","@type":"Researcher","foaf:name":[{"@value":"Ravishankar Narayanan"}],"jpcoar:affiliationName":[{"@value":"Materials Research Centre, Indian Institute of Science, Bangalore 560012, India"}]},{"@id":"https://cir.nii.ac.jp/crid/1380021390742914562","@type":"Researcher","foaf:name":[{"@value":"Matti Knaapila"}],"jpcoar:affiliationName":[{"@value":"Department of Physics, Norwegian University of Science and Technology, 7491 Trondheim, Norway"}]},{"@id":"https://cir.nii.ac.jp/crid/1380021390742914566","@type":"Researcher","foaf:name":[{"@value":"Wakana Matsuda"}],"jpcoar:affiliationName":[{"@value":"Department of Molecular Engineering, Kyoto University, Nishikyo-ku, Kyoto 615-8510, Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380021390742914561","@type":"Researcher","foaf:name":[{"@value":"Shu Seki"}],"jpcoar:affiliationName":[{"@value":"Department of Molecular Engineering, Kyoto University, Nishikyo-ku, Kyoto 615-8510, Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1380021390742914568","@type":"Researcher","foaf:name":[{"@value":"Satish Patil"}],"jpcoar:affiliationName":[{"@value":"Solid State and Structural Chemistry Unit, Indian Institute of Science, Bangalore 560012, India"}]}],"publication":{"publicationIdentifier":[{"@type":"PISSN","@value":"26376113"},{"@type":"EISSN","@value":"26376113"}],"prism:publicationName":[{"@value":"ACS Applied Electronic Materials"}],"dc:publisher":[{"@value":"American Chemical Society (ACS)"}],"prism:publicationDate":"2023-08-25","prism:volume":"5","prism:number":"9","prism:startingPage":"5093","prism:endingPage":"5102"},"reviewed":"false","dc:rights":["https://doi.org/10.15223/policy-029","https://doi.org/10.15223/policy-037","https://doi.org/10.15223/policy-045"],"url":[{"@id":"https://pubs.acs.org/doi/pdf/10.1021/acsaelm.3c00845"}],"createdAt":"2023-08-25","modifiedAt":"2023-09-26","foaf:topic":[{"@id":"https://cir.nii.ac.jp/all?q=photoconductivity","dc:title":"photoconductivity"},{"@id":"https://cir.nii.ac.jp/all?q=supramolecular%20structure","dc:title":"supramolecular structure"},{"@id":"https://cir.nii.ac.jp/all?q=diketopyrrolopyrrole","dc:title":"diketopyrrolopyrrole"},{"@id":"https://cir.nii.ac.jp/all?q=noncovalent%20interaction","dc:title":"noncovalent interaction"},{"@id":"https://cir.nii.ac.jp/all?q=mobility","dc:title":"mobility"},{"@id":"https://cir.nii.ac.jp/all?q=info:eu-repo/classification/ddc/620","dc:title":"info:eu-repo/classification/ddc/620"}],"project":[{"@id":"https://cir.nii.ac.jp/crid/1040567901045566336","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"20H05867"},{"@type":"JGN","@value":"JP20H05867"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PLANNED-20H05867/"}],"notation":[{"@language":"ja","@value":"先端計測技術を用いた高密度共役分子集積体の物性解明"},{"@language":"en","@value":"Elucidation of Physical Properties in High-Density Conjugated Molecular Assemblies Using Advanced Measurement 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