{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1360021390743354240.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1038/s41427-023-00520-w"}},{"identifier":{"@type":"URI","@value":"https://www.nature.com/articles/s41427-023-00520-w.pdf"}},{"identifier":{"@type":"URI","@value":"https://www.nature.com/articles/s41427-023-00520-w"}}],"resourceType":"学術雑誌論文(journal article)","dc:title":[{"@value":"Recent progress in thermoelectric layered cobalt oxide thin films"}],"description":[{"type":"abstract","notation":[{"@value":"<jats:title>Abstract</jats:title><jats:p>Oxide-based thermoelectric materials that show a high figure of merit are promising because of their good chemical and thermal stabilities and their relative harmlessness compared with chalcogenide-based state-of-the-art thermoelectric materials. Although several high-<jats:italic>ZT</jats:italic> thermoelectric oxides (<jats:italic>ZT</jats:italic> > 1) have been reported thus far, their reliability levels are low due to the lack of careful observations of their stabilities at elevated temperatures. Herein, we review the epitaxial film growth and thermoelectric properties of representative p-type layered cobalt oxides: Na<jats:sub>3/4</jats:sub>CoO<jats:sub>2</jats:sub>, Ca<jats:sub>1/3</jats:sub>CoO<jats:sub>2</jats:sub>, Sr<jats:sub>1/3</jats:sub>CoO<jats:sub>2</jats:sub>, Ba<jats:sub>1/3</jats:sub>CoO<jats:sub>2</jats:sub>, and Ca<jats:sub>3</jats:sub>Co<jats:sub>4</jats:sub>O<jats:sub>9</jats:sub>. Among these specimens, Ba<jats:sub>1/3</jats:sub>CoO<jats:sub>2</jats:sub> and Ca<jats:sub>3</jats:sub>Co<jats:sub>4</jats:sub>O<jats:sub>9</jats:sub> are stable in air at elevated temperatures (~600 °C). The <jats:italic>ZT</jats:italic> of Ba<jats:sub>1/3</jats:sub>CoO<jats:sub>2</jats:sub> reaches ~ 0.55 at 600 °C in air, which is reliable and the highest among thermoelectric oxides. Moreover, this value is comparable to those of p-type PbTe and p-type SiGe.</jats:p>"}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1380021390743354126","@type":"Researcher","foaf:name":[{"@value":"Yuqiao Zhang"}]},{"@id":"https://cir.nii.ac.jp/crid/1420001326235996928","@type":"Researcher","personIdentifier":[{"@type":"KAKEN_RESEARCHERS","@value":"80372530"},{"@type":"NRID","@value":"1000080372530"},{"@type":"NRID","@value":"9000022364509"},{"@type":"NRID","@value":"9000413564430"},{"@type":"NRID","@value":"9000411496321"},{"@type":"NRID","@value":"9000402913178"},{"@type":"NRID","@value":"9000415343346"},{"@type":"NRID","@value":"9000006575490"},{"@type":"NRID","@value":"9000239588943"},{"@type":"NRID","@value":"9000239588939"},{"@type":"NRID","@value":"9000022345897"},{"@type":"NRID","@value":"9000023732241"},{"@type":"NRID","@value":"9000414939050"},{"@type":"NRID","@value":"9000413946981"},{"@type":"NRID","@value":"9000397706949"},{"@type":"NRID","@value":"9000023711769"},{"@type":"NRID","@value":"9000411833771"},{"@type":"NRID","@value":"9000399947553"},{"@type":"NRID","@value":"9000412574210"},{"@type":"NRID","@value":"9000279888191"},{"@type":"NRID","@value":"9000381958731"},{"@type":"NRID","@value":"9000409024190"},{"@type":"NRID","@value":"9000389944836"},{"@type":"NRID","@value":"9000391875383"},{"@type":"NRID","@value":"9000401978386"},{"@type":"NRID","@value":"9000388461302"},{"@type":"NRID","@value":"9000107341968"},{"@type":"NRID","@value":"9000023712490"},{"@type":"NRID","@value":"9000414839122"},{"@type":"NRID","@value":"9000326266929"},{"@type":"NRID","@value":"9000022345991"},{"@type":"NRID","@value":"9000022396373"},{"@type":"NRID","@value":"9000413503662"},{"@type":"NRID","@value":"9000303992649"},{"@type":"NRID","@value":"9000403973953"},{"@type":"NRID","@value":"9000411032505"},{"@type":"NRID","@value":"9000023834235"},{"@type":"NRID","@value":"9000414242854"},{"@type":"NRID","@value":"9000411248883"},{"@type":"NRID","@value":"9000398389804"},{"@type":"NRID","@value":"9000411514339"},{"@type":"NRID","@value":"9000267846635"},{"@type":"NRID","@value":"9000239589139"},{"@type":"NRID","@value":"9000239589160"},{"@type":"NRID","@value":"9000239589147"},{"@type":"NRID","@value":"9000414843856"},{"@type":"NRID","@value":"9000412109983"},{"@type":"NRID","@value":"9000000040577"},{"@type":"NRID","@value":"9000412584090"},{"@type":"NRID","@value":"9000403973958"},{"@type":"NRID","@value":"9000277508634"},{"@type":"NRID","@value":"9000391846089"},{"@type":"NRID","@value":"9000401566079"},{"@type":"NRID","@value":"9000336757266"},{"@type":"NRID","@value":"9000398389799"},{"@type":"NRID","@value":"9000406302634"},{"@type":"NRID","@value":"9000290134497"},{"@type":"NRID","@value":"9000402046662"},{"@type":"NRID","@value":"9000024713155"},{"@type":"NRID","@value":"9000024409865"},{"@type":"NRID","@value":"9000388460437"},{"@type":"NRID","@value":"9000414953124"},{"@type":"NRID","@value":"9000239588922"},{"@type":"NRID","@value":"9000411519861"},{"@type":"NRID","@value":"9000409990894"},{"@type":"NRID","@value":"9000401994106"},{"@type":"NRID","@value":"9000258460541"},{"@type":"NRID","@value":"9000023749240"},{"@type":"NRID","@value":"9000326661565"},{"@type":"NRID","@value":"9000411077054"},{"@type":"NRID","@value":"9000362200167"},{"@type":"NRID","@value":"9000401980427"},{"@type":"NRID","@value":"9000381460736"},{"@type":"NRID","@value":"9000257847883"},{"@type":"NRID","@value":"9000023834805"},{"@type":"NRID","@value":"9000414725570"},{"@type":"NRID","@value":"9000413330921"},{"@type":"NRID","@value":"9000411999563"},{"@type":"NRID","@value":"9000360556009"},{"@type":"NRID","@value":"9000345325372"},{"@type":"NRID","@value":"9000401900644"},{"@type":"NRID","@value":"9000023732114"},{"@type":"NRID","@value":"9000409177056"},{"@type":"NRID","@value":"9000414521886"},{"@type":"RESEARCHMAP","@value":"https://researchmap.jp/read0132908"}],"foaf:name":[{"@value":"Hiromichi 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LLC"}],"prism:publicationDate":"2023-12-29","prism:volume":"15","prism:number":"1","prism:startingPage":"67"},"reviewed":"false","dcterms:accessRights":"http://purl.org/coar/access_right/c_abf2","dc:rights":["https://creativecommons.org/licenses/by/4.0","https://creativecommons.org/licenses/by/4.0"],"url":[{"@id":"https://www.nature.com/articles/s41427-023-00520-w.pdf"},{"@id":"https://www.nature.com/articles/s41427-023-00520-w"}],"createdAt":"2023-12-29","modifiedAt":"2024-02-05","project":[{"@id":"https://cir.nii.ac.jp/crid/1040003825673365120","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"19H05791"},{"@type":"JGN","@value":"JP19H05791"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PLANNED-19H05791/"}],"notation":[{"@language":"ja","@value":"界面制御による高機能薄膜材料創製"},{"@language":"en","@value":"Fabrication of highly functional thin film materials by controlling the interface"}]}],"relatedProduct":[{"@id":"https://cir.nii.ac.jp/crid/1050001338795667968","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["references"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Large thermoelectric performance of heavily Nb-doped SrTiO_3 epitaxial film at high temperature"}]},{"@id":"https://cir.nii.ac.jp/crid/1050001338795670144","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["references"],"jpcoar:relatedTitle":[{"@language":"en","@value":"High electrical conductivity of layered cobalt oxide Ca_3Co_4O_9 epitaxial films grown by topotactic ion-exchange method"}]},{"@id":"https://cir.nii.ac.jp/crid/1050025031474855168","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["references"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Anisotropic Heat Conduction in Ion‐Substituted Layered Cobalt Oxides"},{"@value":"Anisotropic heat conduction in ion-substituted layered cobalt 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layered Ba<sub>x</sub>CoO<sub>2</sub>"}]},{"@id":"https://cir.nii.ac.jp/crid/1360294723748017152","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"High performance (ZT>1) n-type oxide thermoelectric composites from earth abundant materials"}]},{"@id":"https://cir.nii.ac.jp/crid/1360302866834724992","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Ba<sub>1/3</sub>CoO<sub>2</sub>: A Thermoelectric Oxide Showing a Reliable <i>ZT</i> of ∼0.55 at 600 °C in Air"}]},{"@id":"https://cir.nii.ac.jp/crid/1360302868779835904","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Enhancement of the thermopower in in the large-x regime ()"}]},{"@id":"https://cir.nii.ac.jp/crid/1360302868780217344","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Preparation and thermoelectric properties of heavily Nb-doped SrO(SrTiO3)1 epitaxial films"}]},{"@id":"https://cir.nii.ac.jp/crid/1360306906087364736","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Synthesis and catalysis of a Co13 disk surrounded by vanadium–oxygen crown"}]},{"@id":"https://cir.nii.ac.jp/crid/1360574093556338176","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Electronic structure of<mml:math xmlns:mml=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=\"normal\">NaCo</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=\"normal\">O</mml:mi></mml:mrow><mml:mrow><mml:mn>4</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>"}]},{"@id":"https://cir.nii.ac.jp/crid/1360574093727618048","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Thermoelectric Behavior of Nickel 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crystals"}]},{"@id":"https://cir.nii.ac.jp/crid/1360855571232803072","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Large enhancement of the thermopower in NaxCoO2 at high Na doping"}]},{"@id":"https://cir.nii.ac.jp/crid/1360857593788172800","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Selective Enhancement in Phonon Scattering Leads to a High Thermoelectric Figure-of-Merit in Graphene Oxide-Encapsulated ZnO Nanocomposites"}]},{"@id":"https://cir.nii.ac.jp/crid/1361137043528755072","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Large thermoelectric response of metallic perovskites:<mml:math xmlns:mml=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=\"normal\">Sr</mml:mi></mml:mrow><mml:mrow><mml:mn>1</mml:mn><mml:mi>−</mml:mi><mml:mi>x</mml:mi></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=\"normal\">La</mml:mi></mml:mrow><mml:mrow><mml:mi>x</mml:mi></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=\"normal\">TiO</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mi> </mml:mi><mml:mo>(</mml:mo><mml:mn>0</mml:mn><mml:mn/><mml:mo><~</mml:mo><mml:mi>x</mml:mi><mml:mo><~</mml:mo><mml:mn>0</mml:mn><mml:mo>.</mml:mo><mml:mn>1</mml:mn><mml:mo>)</mml:mo></mml:math>"}]},{"@id":"https://cir.nii.ac.jp/crid/1361137043765898880","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Electrical Transport Properties and High-Temperature Thermoelectric Performance of (Ca0.9M0.1)MnO3 (M = Y, La, Ce, Sm, In, Sn, Sb, Pb, Bi)"}]},{"@id":"https://cir.nii.ac.jp/crid/1361137044520187776","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Ultralow thermal conductivity and high thermoelectric figure of merit in SnSe crystals"}]},{"@id":"https://cir.nii.ac.jp/crid/1361137045031034624","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Peierls distortion as a route to high thermoelectric performance in In4Se3-δ crystals"}]},{"@id":"https://cir.nii.ac.jp/crid/1361137045194129280","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"High-temperature thermoelectric properties of (Zn1−<i>x</i>Al<i>x</i>)O"}]},{"@id":"https://cir.nii.ac.jp/crid/1361418518552116992","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Spin entropy as the likely source of enhanced thermopower in 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