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Previous studies have assumed no interactions between organic aerosols and liquid CH<jats:sub>4</jats:sub>, although the dissolution of low‐molecular‐weight photochemical products in liquid CH<jats:sub>4</jats:sub> has been considered. Here we report experimental results of soaking a laboratory analog (so‐called tholin) of Titan's organic aerosols in liquid CH<jats:sub>4</jats:sub> at 93–98 K for several hours and then evaporating the liquid, simulating wet–dry cycling on Titan. After wet–dry cycling, residual tholin particles form aggregates through cementation. Solid evaporitic deposits formed by evaporation of interacted liquid contain nitrogen‐bearing aromatics, suggesting selective dissolution of aromatics. Our results suggest that organic aerosols or high‐molecular‐weight compounds adsorbed on them partly dissolve in liquid CH<jats:sub>4</jats:sub> on Titan, even during short‐term wetting events, promoting the growth of aerosols to dune particles via aggregation and providing aromatics to evaporites.</jats:p>"}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1380021391860607492","@type":"Researcher","foaf:name":[{"@value":"Eito Hirai"}],"jpcoar:affiliationName":[{"@value":"Earth–Life Science Institute (ELSI) Tokyo Institute of Technology  Tokyo Japan"},{"@value":"Department of Earth and Planetary Science Tokyo Institute of Technology  Tokyo 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Cosmic physics"},{"@id":"https://cir.nii.ac.jp/all?q=organic%20aerosols","dc:title":"organic aerosols"},{"@id":"https://cir.nii.ac.jp/all?q=hydrocarbons","dc:title":"hydrocarbons"},{"@id":"https://cir.nii.ac.jp/all?q=Titan","dc:title":"Titan"},{"@id":"https://cir.nii.ac.jp/all?q=geochemical%20processes","dc:title":"geochemical processes"},{"@id":"https://cir.nii.ac.jp/all?q=tholins","dc:title":"tholins"}],"project":[{"@id":"https://cir.nii.ac.jp/crid/1040003825717557632","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"20H00195"},{"@type":"JGN","@value":"JP20H00195"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-20H00195/"}],"notation":[{"@language":"ja","@value":"地下凍土融解地域の地質・微生物調査及び機械学習に基づく火星水環境の理解"},{"@language":"en","@value":"Martian aqueous environments from geological and microbiological surveys of ground ice regions and machine learning"}]},{"@id":"https://cir.nii.ac.jp/crid/1040014327101519744","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"23H00144"},{"@type":"JGN","@value":"JP23H00144"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-23H00144/"}],"notation":[{"@language":"ja","@value":"太陽系氷天体の海洋化学と有機化学進化の実験理論予測"},{"@language":"en","@value":"Experimental and theoretical predictions of ocean chemistry and organic chemical evolution of icy bodies in the Solar System"}]},{"@id":"https://cir.nii.ac.jp/crid/1040288757437886208","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"21K18917"},{"@type":"JGN","@value":"JP21K18917"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-21K18917/"}],"notation":[{"@language":"ja","@value":"粘土鉱物により放射性核種は還元されるか？ -放射性廃棄物地層処分と関連して-"},{"@language":"en","@value":"Are radionuclides reduced by clay minerals? 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