{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1360848657448304512.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1016/j.susc.2013.08.010"}},{"identifier":{"@type":"URI","@value":"https://api.elsevier.com/content/article/PII:S0039602813002355?httpAccept=text/xml"}},{"identifier":{"@type":"URI","@value":"https://api.elsevier.com/content/article/PII:S0039602813002355?httpAccept=text/plain"}}],"resourceType":"学術雑誌論文(journal article)","dc:title":[{"@value":"Tip-enhanced Raman spectroscopy of 4,4′-bipyridine and 4,4′-bipyridine N,N'-dioxide adsorbed on gold thin films"}],"description":[{"notation":[{"@value":"Abstract   A tip-enhanced Raman spectroscopy (TERS) set-up added on a scanning tunneling microscope (STM) was constructed and was used to study the molecular arrangement of 4,4′-bipyridine (4,4′-BiPy) and 4,4′-bipyridine  N,N' -dioxide (4,4′-BiPyO 2 ) adsorbed on Au(111). Over a monolayer of 4,4′-BiPy, in the ambient atmosphere, intense TERS signals were recorded, involving Au N stretching vibration at 185 cm − 1 . At the early stage of 4,4′-BiPy adsorption, the Au N stretching signal was not detected. By the aid of the theoretical calculations of the Raman scattering intensities for each vibrational normal mode, a standing-up, tilted orientation at monolayer coverage and a vertical orientation with the longitudinal molecular axis parallel to the surface at low surface coverage was concluded. Adsorption of 4,4′-BiPyO 2  on Au(111) resulted in formation of a (6 × 9) adlattice. Moderately intense TERS signals were observed, containing the N O stretching modes and the in-plane ring vibrational modes. Neither Au O nor Au N stretching modes were observed. 4,4′-BiPyO 2  was laid with the longitudinal axis parallel to the surface, and the molecular plane vertical to the surface. These results demonstrate that STM-TERS is an effective method for simultaneous imaging and vibrational analysis, facilitating identification of the adsorbed layers with the nanometer-scale spatial resolution and monolayer sensitivity."}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1380848657448304516","@type":"Researcher","foaf:name":[{"@value":"I.I. Rzeźnicka"}]},{"@id":"https://cir.nii.ac.jp/crid/1380848657448304514","@type":"Researcher","foaf:name":[{"@value":"H. Horino"}]},{"@id":"https://cir.nii.ac.jp/crid/1380848657448304513","@type":"Researcher","foaf:name":[{"@value":"N. Kikkawa"}]},{"@id":"https://cir.nii.ac.jp/crid/1380848657448304515","@type":"Researcher","foaf:name":[{"@value":"S. Sakaguchi"}]},{"@id":"https://cir.nii.ac.jp/crid/1380848657448304517","@type":"Researcher","foaf:name":[{"@value":"A. Morita"}]},{"@id":"https://cir.nii.ac.jp/crid/1380848657448304519","@type":"Researcher","foaf:name":[{"@value":"S. Takahashi"}]},{"@id":"https://cir.nii.ac.jp/crid/1380848657448304518","@type":"Researcher","foaf:name":[{"@value":"T. Komeda"}]},{"@id":"https://cir.nii.ac.jp/crid/1380848657448304520","@type":"Researcher","foaf:name":[{"@value":"H. Fukumura"}]},{"@id":"https://cir.nii.ac.jp/crid/1380848657448304512","@type":"Researcher","foaf:name":[{"@value":"T. Yamada"}]},{"@id":"https://cir.nii.ac.jp/crid/1380848657448304521","@type":"Researcher","foaf:name":[{"@value":"M. Kawai"}]}],"publication":{"publicationIdentifier":[{"@type":"PISSN","@value":"00396028"}],"prism:publicationName":[{"@value":"Surface Science"}],"dc:publisher":[{"@value":"Elsevier BV"}],"prism:publicationDate":"2013-11","prism:volume":"617","prism:startingPage":"1","prism:endingPage":"9"},"reviewed":"false","invited":"false","dc:rights":["https://www.elsevier.com/tdm/userlicense/1.0/","https://www.elsevier.com/legal/tdmrep-license"],"url":[{"@id":"https://api.elsevier.com/content/article/PII:S0039602813002355?httpAccept=text/xml"},{"@id":"https://api.elsevier.com/content/article/PII:S0039602813002355?httpAccept=text/plain"}],"createdAt":"2013-08-17","modifiedAt":"2025-09-22","project":[{"@id":"https://cir.nii.ac.jp/crid/1040000782065723520","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"21245002"},{"@type":"JGN","@value":"JP21245002"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-21245002/"}],"notation":[{"@language":"ja","@value":"界面和周波分光の理論計算手法の開発と応用"},{"@language":"en","@value":"Theory and computational method of interfacial sum frequency generation spectrosocpy"}]},{"@id":"https://cir.nii.ac.jp/crid/1040000782234038016","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"25104007"},{"@type":"JGN","@value":"JP25104007"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PLANNED-25104007/"}],"notation":[{"@language":"ja","@value":"高度化した一分子蛍光計測によるタンパク質の構造形成運動の解明"},{"@language":"en","@value":"Investigation on the dynamics of protein folding by single molecule fluorescence spectroscopy"}]},{"@id":"https://cir.nii.ac.jp/crid/1040000782436746880","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"13J02345"},{"@type":"JGN","@value":"JP13J02345"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-13J02345/"}],"notation":[{"@language":"ja","@value":"界面の分子科学を基礎とした相間移動触媒反応のマルチスケールシミュレーション"}]},{"@id":"https://cir.nii.ac.jp/crid/1040282257210715904","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"25104003"},{"@type":"JGN","@value":"JP25104003"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PLANNED-25104003/"}],"notation":[{"@language":"ja","@value":"溶液・高分子系界面の構造および機能の理論解析"},{"@language":"en","@value":"Theory of Structure and Functions of Liquid and Polymer Interfaces"}]},{"@id":"https://cir.nii.ac.jp/crid/1040282257229786368","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"25390001"},{"@type":"JGN","@value":"JP25390001"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-25390001/"}],"notation":[{"@language":"ja","@value":"Fabrication of plasmonic metal nano-structures for photocurrent generation drawing an innovation for design of thin-film solar cells"},{"@language":"en","@value":"Fabrication of plasmonic metal nano-structures for photocurrent generation drawing an innovation for design of thin-film solar cells"}]}],"relatedProduct":[{"@id":"https://cir.nii.ac.jp/crid/1050025031473789312","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Room-Temperature Molecular Manipulation via Plasmonic Trapping at Electrified Interfaces"}]},{"@id":"https://cir.nii.ac.jp/crid/1360002215276141696","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Tip-enhanced THz Raman spectroscopy for local temperature determination at the nanoscale"}]},{"@id":"https://cir.nii.ac.jp/crid/1360011143793319680","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Adsorption characteristics of 4,4′-bipyridine molecules on gold nanosphere films studied by surface-enhanced Raman scattering"}]},{"@id":"https://cir.nii.ac.jp/crid/1360011144018689792","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Adsorbed Structures of 4,4‘-Bipyridine on Cu(111) in Acid Studied by STM and IR"}]},{"@id":"https://cir.nii.ac.jp/crid/1360011144114384256","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Tip-Enhanced Raman Spectroscopy Can See More:  The Case of Cytochrome c"}]},{"@id":"https://cir.nii.ac.jp/crid/1360011145381756544","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Studying Surface Chemistry beyond the Diffraction Limit: 10 Years of TERS"}]},{"@id":"https://cir.nii.ac.jp/crid/1360292618802009984","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Interactions between organized, surface-confined monolayers and vapor-phase probe molecules. 7. 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