{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1361418520828519936.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1126/science.1135941"}},{"identifier":{"@type":"URI","@value":"https://www.science.org/doi/pdf/10.1126/science.1135941"}}],"dc:title":[{"@value":"Improved Oxygen Reduction Activity on Pt\n            <sub>3</sub>\n            Ni(111) via Increased Surface Site Availability"}],"description":[{"type":"abstract","notation":[{"@value":"<jats:p>\n            The slow rate of the oxygen reduction reaction (ORR) in the polymer electrolyte membrane fuel cell (PEMFC) is the main limitation for automotive applications. We demonstrated that the Pt\n            <jats:sub>3</jats:sub>\n            Ni(111) surface is 10-fold more active for the ORR than the corresponding Pt(111) surface and 90-fold more active than the current state-of-the-art Pt/C catalysts for PEMFC. The Pt\n            <jats:sub>3</jats:sub>\n            Ni(111) surface has an unusual electronic structure (\n            <jats:italic>d</jats:italic>\n            -band center position) and arrangement of surface atoms in the near-surface region. Under operating conditions relevant to fuel cells, its near-surface layer exhibits a highly structured compositional oscillation in the outermost and third layers, which are Pt-rich, and in the second atomic layer, which is Ni-rich. The weak interaction between the Pt surface atoms and nonreactive oxygenated species increases the number of active sites for O\n            <jats:sub>2</jats:sub>\n            adsorption.\n          </jats:p>"}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1381418520828519810","@type":"Researcher","foaf:name":[{"@value":"Vojislav R. Stamenkovic"}],"jpcoar:affiliationName":[{"@value":"Materials Science Division, Argonne National Laboratory, Argonne, IL 60439, USA."},{"@value":"Materials Sciences Division, Lawrence Berkeley National Laboratory, University of California, Berkeley, CA 94720, USA."},{"@value":"Oliver Lodge Laboratory, Department of Physics, University of Liverpool, Liverpool, L69 7ZE, UK."},{"@value":"Department of Chemistry and Physics, University of South Carolina, Aiken, SC 29801, USA."}]},{"@id":"https://cir.nii.ac.jp/crid/1381418520828519812","@type":"Researcher","foaf:name":[{"@value":"Ben Fowler"}],"jpcoar:affiliationName":[{"@value":"Materials Science Division, Argonne National Laboratory, Argonne, IL 60439, USA."},{"@value":"Materials Sciences Division, Lawrence Berkeley National Laboratory, University of California, Berkeley, CA 94720, USA."},{"@value":"Oliver Lodge Laboratory, Department of Physics, University of Liverpool, Liverpool, L69 7ZE, UK."},{"@value":"Department of Chemistry and Physics, University of South Carolina, Aiken, SC 29801, USA."}]},{"@id":"https://cir.nii.ac.jp/crid/1381418520828519811","@type":"Researcher","foaf:name":[{"@value":"Bongjin Simon Mun"}],"jpcoar:affiliationName":[{"@value":"Materials Science Division, Argonne National Laboratory, Argonne, IL 60439, USA."},{"@value":"Materials Sciences Division, Lawrence Berkeley National Laboratory, University of California, Berkeley, CA 94720, USA."},{"@value":"Oliver Lodge Laboratory, Department of Physics, University of Liverpool, Liverpool, L69 7ZE, UK."},{"@value":"Department of Chemistry and Physics, University of South Carolina, Aiken, SC 29801, USA."}]},{"@id":"https://cir.nii.ac.jp/crid/1381418520828519808","@type":"Researcher","foaf:name":[{"@value":"Guofeng Wang"}],"jpcoar:affiliationName":[{"@value":"Materials Science Division, Argonne National Laboratory, Argonne, IL 60439, USA."},{"@value":"Materials Sciences Division, Lawrence Berkeley National Laboratory, University of California, Berkeley, CA 94720, USA."},{"@value":"Oliver Lodge Laboratory, Department of Physics, University of Liverpool, Liverpool, L69 7ZE, UK."},{"@value":"Department of Chemistry and Physics, University of South Carolina, Aiken, SC 29801, USA."}]},{"@id":"https://cir.nii.ac.jp/crid/1381418520828519813","@type":"Researcher","foaf:name":[{"@value":"Philip N. Ross"}],"jpcoar:affiliationName":[{"@value":"Materials Science Division, Argonne National Laboratory, Argonne, IL 60439, USA."},{"@value":"Materials Sciences Division, Lawrence Berkeley National Laboratory, University of California, Berkeley, CA 94720, USA."},{"@value":"Oliver Lodge Laboratory, Department of Physics, University of Liverpool, Liverpool, L69 7ZE, UK."},{"@value":"Department of Chemistry and Physics, University of South Carolina, Aiken, SC 29801, USA."}]},{"@id":"https://cir.nii.ac.jp/crid/1381418520828519936","@type":"Researcher","foaf:name":[{"@value":"Christopher A. Lucas"}],"jpcoar:affiliationName":[{"@value":"Materials Science Division, Argonne National Laboratory, Argonne, IL 60439, USA."},{"@value":"Materials Sciences Division, Lawrence Berkeley National Laboratory, University of California, Berkeley, CA 94720, USA."},{"@value":"Oliver Lodge Laboratory, Department of Physics, University of Liverpool, Liverpool, L69 7ZE, UK."},{"@value":"Department of Chemistry and Physics, University of South Carolina, Aiken, SC 29801, USA."}]},{"@id":"https://cir.nii.ac.jp/crid/1381418520828519809","@type":"Researcher","foaf:name":[{"@value":"Nenad M. Marković"}],"jpcoar:affiliationName":[{"@value":"Materials Science Division, Argonne National Laboratory, Argonne, IL 60439, USA."},{"@value":"Materials Sciences Division, Lawrence Berkeley National Laboratory, University of California, Berkeley, CA 94720, USA."},{"@value":"Oliver Lodge Laboratory, Department of Physics, University of Liverpool, Liverpool, L69 7ZE, UK."},{"@value":"Department of Chemistry and Physics, University of South Carolina, Aiken, SC 29801, USA."}]}],"publication":{"publicationIdentifier":[{"@type":"PISSN","@value":"00368075"},{"@type":"EISSN","@value":"10959203"}],"prism:publicationName":[{"@value":"Science"}],"dc:publisher":[{"@value":"American Association for the Advancement of Science (AAAS)"}],"prism:publicationDate":"2007-01-26","prism:volume":"315","prism:number":"5811","prism:startingPage":"493","prism:endingPage":"497"},"reviewed":"false","url":[{"@id":"https://www.science.org/doi/pdf/10.1126/science.1135941"}],"createdAt":"2007-01-12","modifiedAt":"2024-01-10","relatedProduct":[{"@id":"https://cir.nii.ac.jp/crid/1050008688836899200","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Ultrafine Pt–Ni nanoparticles in hollow porous carbon spheres for remarkable oxygen reduction reaction catalysis"}]},{"@id":"https://cir.nii.ac.jp/crid/1050014713339766400","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Stabilization of unprecedented crystal phases of metal nanomaterials"}]},{"@id":"https://cir.nii.ac.jp/crid/1050306506452946688","@type":"Article","resourceType":"学術雑誌論文(journal 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