{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1361699993623831808.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1038/nchem.1655"}},{"identifier":{"@type":"URI","@value":"http://www.nature.com/articles/nchem.1655.pdf"}},{"identifier":{"@type":"URI","@value":"http://www.nature.com/articles/nchem.1655"}},{"identifier":{"@type":"PMID","@value":"23787746"}}],"dc:title":[{"@value":"Initiation of carbon nanotube growth by well-defined carbon nanorings"}],"description":[{"notation":[{"@value":"Carbon nanotubes (CNTs), tubular molecular entities that consist of sp(2)-hybridized carbon atoms, are currently produced as mixtures that contain tubes of various diameters and different sidewall structures. The electronic and optical properties of CNTs are determined by their diameters and sidewall structures and so a controlled synthesis of uniform-diameter, single-chirality CNTs-a significant chemical challenge-would provide access to pure samples with predictable properties. Here we report a rational bottom-up approach to synthesize structurally uniform CNTs using carbon nanorings (cycloparaphenylenes) as templates and ethanol as the carbon source. The average diameter of the CNTs formed is close to that of the carbon nanorings used, which supports the operation of a 'growth-from-template' mechanism in CNT formation. This bottom-up organic chemistry approach is intrinsically different from other conventional approaches to making CNTs and, if it can be optimized sufficiently, offers a route to the programmable synthesis of structurally uniform CNTs."}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1381699993623831811","@type":"Researcher","foaf:name":[{"@value":"Haruka Omachi"}]},{"@id":"https://cir.nii.ac.jp/crid/1381699993623831812","@type":"Researcher","foaf:name":[{"@value":"Takuya Nakayama"}]},{"@id":"https://cir.nii.ac.jp/crid/1381699993623831809","@type":"Researcher","foaf:name":[{"@value":"Eri Takahashi"}]},{"@id":"https://cir.nii.ac.jp/crid/1381699993623831810","@type":"Researcher","foaf:name":[{"@value":"Yasutomo Segawa"}]},{"@id":"https://cir.nii.ac.jp/crid/1381699993623831808","@type":"Researcher","foaf:name":[{"@value":"Kenichiro Itami"}]}],"publication":{"publicationIdentifier":[{"@type":"PISSN","@value":"17554330"},{"@type":"EISSN","@value":"17554349"}],"prism:publicationName":[{"@value":"Nature Chemistry"}],"dc:publisher":[{"@value":"Springer Science and Business Media LLC"}],"prism:publicationDate":"2013-05-26","prism:volume":"5","prism:number":"7","prism:startingPage":"572","prism:endingPage":"576"},"reviewed":"false","dc:rights":["http://www.springer.com/tdm"],"url":[{"@id":"http://www.nature.com/articles/nchem.1655.pdf"},{"@id":"http://www.nature.com/articles/nchem.1655"}],"createdAt":"2013-05-24","modifiedAt":"2023-05-18","foaf:topic":[{"@id":"https://cir.nii.ac.jp/all?q=Spectrometry,%20Fluorescence","dc:title":"Spectrometry, Fluorescence"},{"@id":"https://cir.nii.ac.jp/all?q=Spectrophotometry,%20Infrared","dc:title":"Spectrophotometry, Infrared"},{"@id":"https://cir.nii.ac.jp/all?q=Nanotubes,%20Carbon","dc:title":"Nanotubes, Carbon"},{"@id":"https://cir.nii.ac.jp/all?q=Stereoisomerism","dc:title":"Stereoisomerism"},{"@id":"https://cir.nii.ac.jp/all?q=Spectrum%20Analysis,%20Raman","dc:title":"Spectrum Analysis, Raman"}],"relatedProduct":[{"@id":"https://cir.nii.ac.jp/crid/1050001338813802112","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Synthesis and Size-Dependent Properties of [12], [16], and [24]Carbon Nanobelts"}]},{"@id":"https://cir.nii.ac.jp/crid/1050564285802716416","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@language":"en","@value":"The Raman fingerprint of cyclic conjugation: the case of the stabilization of cations and dications in cycloparaphenylenes"}]},{"@id":"https://cir.nii.ac.jp/crid/1050580605009672960","@type":"Article","resourceType":"学術雑誌論文(journal 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σ-Bonds Leading to an Efficient Synthesis of [\n                    <i>n</i>\n                    ]Cycloparaphenylenes (\n                    <i>n</i>\n                    = 9–15) by Self-Assembly"}]},{"@id":"https://cir.nii.ac.jp/crid/1360025439745635200","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Synthesis of Cyclophenacene‐ and Chiral‐Type Cyclophenylene‐Naphthylene Belts"}]},{"@id":"https://cir.nii.ac.jp/crid/1360283689401292032","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Synthesis, Characterization, and Properties of [4]Cyclo‐2,7‐pyrenylene: Effects of Cyclic Structure on the Electronic Properties of Pyrene Oligomers"}]},{"@id":"https://cir.nii.ac.jp/crid/1360283692409819776","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Insights into 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1,4‐Dihydroxycyclo‐2,5‐diene Precursors"}]},{"@id":"https://cir.nii.ac.jp/crid/1360565166612180864","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Synthesis and Characterization of [5]Cycloparaphenylene"}]},{"@id":"https://cir.nii.ac.jp/crid/1360565166750807808","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Structurally uniform and atomically precise carbon nanostructures"}]},{"@id":"https://cir.nii.ac.jp/crid/1360567179876036224","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Design and Synthesis of Carbon Nanotube Segments"}]},{"@id":"https://cir.nii.ac.jp/crid/1360567179947530752","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Nonplanar Butterfly‐Shaped π‐Expanded 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