{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1361975845803845248.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1126/science.aax8018"}},{"identifier":{"@type":"URI","@value":"https://syndication.highwire.org/content/doi/10.1126/science.aax8018"}},{"identifier":{"@type":"URI","@value":"https://www.science.org/doi/pdf/10.1126/science.aax8018"}}],"resourceType":"学術雑誌論文(journal article)","dc:title":[{"@value":"Stabilizing heterostructures of soft perovskite semiconductors"}],"description":[{"type":"abstract","notation":[{"@value":"<jats:title>Strong perovskite interfaces</jats:title>\n          <jats:p>\n            The weak bonding in the crystal lattice of hybrid perovskites used in solar cells promotes surface decomposition and interferes with the formation of stable heterostructures with the charge carrier layers. Y. Wang\n            <jats:italic>et al.</jats:italic>\n            show that strong bonds are formed between lead and both chlorine and oxygen atoms in a film with a lead-rich surface and a chlorinated graphene oxide layer. This interface was used with common hole-transporting materials to fabricate solar cells that maintained 90% of their initial efficiency of 21% after operation at 60°C for 1000 hours.\n          </jats:p>\n          <jats:p>\n            <jats:italic>Science</jats:italic>\n            , this issue p.\n            <jats:related-article xmlns:xlink=\"http://www.w3.org/1999/xlink\" ext-link-type=\"doi\" issue=\"6454\" page=\"687\" related-article-type=\"in-this-issue\" vol=\"365\" xlink:href=\"10.1126/science.aax8018\">687</jats:related-article>\n          </jats:p>"}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1381975845803845508","@type":"Researcher","foaf:name":[{"@value":"Yanbo Wang"}],"jpcoar:affiliationName":[{"@value":"State Key Laboratory of Metal Matrix Composites, Shanghai Jiao Tong University, Shanghai 200240, China."}]},{"@id":"https://cir.nii.ac.jp/crid/1381975845803845376","@type":"Researcher","foaf:name":[{"@value":"Tianhao Wu"}],"jpcoar:affiliationName":[{"@value":"State Key Laboratory of Metal Matrix Composites, Shanghai Jiao Tong University, Shanghai 200240, China."}]},{"@id":"https://cir.nii.ac.jp/crid/1381975845803845507","@type":"Researcher","foaf:name":[{"@value":"Julien Barbaud"}],"jpcoar:affiliationName":[{"@value":"State Key Laboratory of Metal Matrix Composites, Shanghai Jiao Tong University, Shanghai 200240, China."}]},{"@id":"https://cir.nii.ac.jp/crid/1381975845803845504","@type":"Researcher","foaf:name":[{"@value":"Weiyu Kong"}],"jpcoar:affiliationName":[{"@value":"State Key Laboratory of Metal Matrix Composites, Shanghai Jiao Tong University, Shanghai 200240, China."}]},{"@id":"https://cir.nii.ac.jp/crid/1381975845803845509","@type":"Researcher","foaf:name":[{"@value":"Danyu Cui"}],"jpcoar:affiliationName":[{"@value":"State Key Laboratory of Metal Matrix Composites, Shanghai Jiao Tong University, Shanghai 200240, China."}]},{"@id":"https://cir.nii.ac.jp/crid/1381975845803845377","@type":"Researcher","foaf:name":[{"@value":"Han Chen"}],"jpcoar:affiliationName":[{"@value":"State Key Laboratory of Metal Matrix Composites, Shanghai Jiao Tong University, Shanghai 200240, China."}]},{"@id":"https://cir.nii.ac.jp/crid/1381975845803845506","@type":"Researcher","foaf:name":[{"@value":"Xudong Yang"}],"jpcoar:affiliationName":[{"@value":"State Key Laboratory of Metal Matrix Composites, Shanghai Jiao Tong University, Shanghai 200240, China."},{"@value":"Center of Hydrogen Science, School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China."}]},{"@id":"https://cir.nii.ac.jp/crid/1420282801184142208","@type":"Researcher","personIdentifier":[{"@type":"KAKEN_RESEARCHERS","@value":"20531172"},{"@type":"NRID","@value":"1000020531172"}],"foaf:name":[{"@value":"Liyuan Han"}],"jpcoar:affiliationName":[{"@value":"State Key Laboratory of Metal Matrix Composites, Shanghai Jiao Tong University, Shanghai 200240, China."},{"@value":"Center of Hydrogen Science, School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China."},{"@value":"Photovoltaic Materials Group, Center for Green Research on Energy and Environmental Materials, National Institute for Materials Science, Tsukuba, Ibaraki 305-0047, Japan."}]}],"publication":{"publicationIdentifier":[{"@type":"PISSN","@value":"00368075"},{"@type":"EISSN","@value":"10959203"}],"prism:publicationName":[{"@value":"Science"}],"dc:publisher":[{"@value":"American Association for the Advancement of Science (AAAS)"}],"prism:publicationDate":"2019-08-16","prism:volume":"365","prism:number":"6454","prism:startingPage":"687","prism:endingPage":"691"},"reviewed":"false","url":[{"@id":"https://syndication.highwire.org/content/doi/10.1126/science.aax8018"},{"@id":"https://www.science.org/doi/pdf/10.1126/science.aax8018"}],"createdAt":"2019-08-15","modifiedAt":"2024-01-15","project":[{"@id":"https://cir.nii.ac.jp/crid/1040282256969727616","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"18H02078"},{"@type":"JGN","@value":"JP18H02078"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-18H02078/"}],"notation":[{"@language":"ja","@value":"逆型ペロブスカイト太陽電池の発電メカニズムの解明"},{"@language":"en","@value":"Mechnism of Perovskite Solar Cells"}]}],"relatedProduct":[{"@id":"https://cir.nii.ac.jp/crid/1050298975368609920","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Constructing Heterostructure through Bidentate Coordination toward Operationally Stable Inverted Perovskite Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1050301607087216256","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Self‐Assembled Monolayer Hole‐Selective Contact for Up‐Scalable and Cost‐Effective Inverted Perovskite Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1050854882644083840","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Heterogeneous FASnI3 Absorber with Enhanced Electric Field for High-Performance Lead-Free Perovskite Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1050857977639970304","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Elimination of light-induced degradation at the nickel oxide-perovskite heterojunction by aprotic sulfonium layers towards long-term operationally stable inverted perovskite solar cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1360001113993116928","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Graphene oxide as a promising photocatalyst for CO<sub>2</sub>to methanol conversion"}]},{"@id":"https://cir.nii.ac.jp/crid/1360005517145609600","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"How far are we from attaining 10-year lifetime for metal halide perovskite solar cells?"}]},{"@id":"https://cir.nii.ac.jp/crid/1360011143658672384","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Mixed halide hybrid perovskites: a paradigm shift in photovoltaics"}]},{"@id":"https://cir.nii.ac.jp/crid/1360011144163677568","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Graphene oxide as dual functional interface modifier for improving wettability and retarding recombination in hybrid perovskite solar cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1360284924860237440","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Accurate and fast evaluation of perovskite solar cells with least hysteresis"}]},{"@id":"https://cir.nii.ac.jp/crid/1360290617528485504","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Lead-free tin perovskite solar cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1360290617528939008","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Templated growth of FASnI<sub>3</sub> crystals for efficient tin perovskite solar cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1360292619665737856","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"6.5% efficient perovskite quantum-dot-sensitized solar cell"}]},{"@id":"https://cir.nii.ac.jp/crid/1360298755633281664","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Interface Energy‐Level Management toward Efficient Tin Perovskite Solar Cells with Hole‐Transport‐Layer‐Free Structure"}]},{"@id":"https://cir.nii.ac.jp/crid/1360298757410439808","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Overview and Outlook on Graphene and Carbon Nanotubes in Perovskite Photovoltaics from Single‐Junction to Tandem Applications"}]},{"@id":"https://cir.nii.ac.jp/crid/1360572092504659584","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"The Application of Graphene Derivatives in Perovskite Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1360574093882850432","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Elucidating the charge carrier separation and working mechanism of CH3NH3PbI3−xClx perovskite solar cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1360574094148872064","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Relationship between ion migration and interfacial degradation of CH3NH3PbI3 perovskite solar cells under thermal conditions"}]},{"@id":"https://cir.nii.ac.jp/crid/1360574096541634560","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Origin of <i><i>J</i>–<i>V</i></i> Hysteresis in Perovskite Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1360584339772642432","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Study of the Heat‐Induced Degradation Mechanism in PbI<sub>2</sub>‐Excess Perovskite Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1360853567482221440","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Efficient and stable tin perovskite solar cells enabled by amorphous-polycrystalline structure"}]},{"@id":"https://cir.nii.ac.jp/crid/1360853567482370304","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Efficiency progress of inverted perovskite solar cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1360861705593716480","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Reduction of Nonradiative Loss in Inverted Perovskite Solar Cells by Donor−π–Acceptor Dipoles"}]},{"@id":"https://cir.nii.ac.jp/crid/1360861707147114624","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Defect Passivation for Perovskite Solar Cells: from Molecule Design to Device Performance"}]},{"@id":"https://cir.nii.ac.jp/crid/1360869855582456320","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Lattice Matching Anchoring of Hole‐Selective Molecule on Halide Perovskite Surfaces for n‐i‐p Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1361131418420160896","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@value":"Highly efficient tin perovskite solar cells achieved in a wide oxygen concentration range"}]},{"@id":"https://cir.nii.ac.jp/crid/1361137044881218176","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Organometal Halide Perovskites as Visible-Light Sensitizers for Photovoltaic Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1361137046208428160","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Surface passivation of perovskite film for efficient solar cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1361418519824344448","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Control of Electrical Potential Distribution for High-Performance Perovskite Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1361418519873155200","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Covalently Modified Graphene Oxide and Polymer of Intrinsic Microporosity (PIM-1) in Mixed Matrix Thin-Film Composite Membranes"}]},{"@id":"https://cir.nii.ac.jp/crid/1361699994282721280","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"CH<sub>3</sub>NH<sub>3</sub>PbI<sub>3</sub> Perovskite/Fullerene Planar‐Heterojunction Hybrid Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1361699996500784768","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Mobile-Ion-Induced Degradation of Organic Hole-Selective Layers in Perovskite Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1361981469851547904","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Large tunable photoeffect on ion conduction in halide perovskites and implications for photodecomposition"}]},{"@id":"https://cir.nii.ac.jp/crid/1361981469855368704","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Multifunctional Fullerene Derivative for Interface Engineering in Perovskite Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1361981470931198080","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Reliable Measurement of Perovskite Solar Cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1362262944207157120","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"QUANTUM ESPRESSO: a modular and open-source software project for quantum simulations of materials"}]},{"@id":"https://cir.nii.ac.jp/crid/1362262944790217472","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Preparation of Graphitic Oxide"}]},{"@id":"https://cir.nii.ac.jp/crid/1362544418752324352","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Enhanced photovoltage for inverted planar heterojunction perovskite solar cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1362544421418944128","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Interpretation and evolution of open-circuit voltage, recombination, ideality factor and subgap defect states during reversible light-soaking and irreversible degradation of perovskite solar cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1362825894262340352","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Efficient Hybrid Solar Cells Based on Meso-Superstructured Organometal Halide Perovskites"}]},{"@id":"https://cir.nii.ac.jp/crid/1362825895937991168","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Investigating charge dynamics in halide perovskite-sensitized mesostructured solar cells"}]},{"@id":"https://cir.nii.ac.jp/crid/1363107369583177344","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Restoring the Density-Gradient Expansion for Exchange in Solids and Surfaces"}]},{"@id":"https://cir.nii.ac.jp/crid/1363107370908223872","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Perovskite solar cells with 18.21% efficiency and area over 1 cm2 fabricated by heterojunction engineering"}]},{"@id":"https://cir.nii.ac.jp/crid/1363107371147068672","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Air-Exposure Induced Dopant Redistribution and Energy Level Shifts in Spin-Coated Spiro-MeOTAD Films"}]},{"@id":"https://cir.nii.ac.jp/crid/1363388843280875264","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Toward high-efficiency, hysteresis-less, stable perovskite solar cells: unusual doping of a hole-transporting material using a fluorine-containing hydrophobic Lewis acid"}]},{"@id":"https://cir.nii.ac.jp/crid/1363388843563489664","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Highly efficient organic photovoltaic devices utilizing work-function tuned graphene oxide derivatives as the anode and cathode charge extraction layers"}]},{"@id":"https://cir.nii.ac.jp/crid/1363388845597218432","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Density functional perturbation theory for gated two-dimensional heterostructures: Theoretical developments and application to flexural phonons in graphene"}]},{"@id":"https://cir.nii.ac.jp/crid/1363670318430744832","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Cation-Induced Band-Gap Tuning in Organohalide Perovskites: Interplay of Spin–Orbit Coupling and Octahedra Tilting"}]},{"@id":"https://cir.nii.ac.jp/crid/1363670319978427904","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Hydrogen Bonding and Stability of Hybrid Organic–Inorganic Perovskites"}]},{"@id":"https://cir.nii.ac.jp/crid/1363951793220677120","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Revealing the role of organic cations in hybrid halide perovskite CH3NH3PbI3"}]},{"@id":"https://cir.nii.ac.jp/crid/1363951794371943040","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Lead Iodide Perovskite Sensitized All-Solid-State Submicron Thin Film Mesoscopic Solar Cell with Efficiency Exceeding 9%"}]},{"@id":"https://cir.nii.ac.jp/crid/1363951795771144064","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Determination of energy level alignment at interfaces of hybrid and organic solar cells under ambient environment"}]},{"@id":"https://cir.nii.ac.jp/crid/1363951795862373504","@type":"Article","relationType":["references"],"jpcoar:relatedTitle":[{"@value":"Green synthesis of near infrared core/shell quantum dots for photocatalytic hydrogen production"}]}],"dataSourceIdentifier":[{"@type":"CROSSREF","@value":"10.1126/science.aax8018"},{"@type":"KAKEN","@value":"PRODUCT-22951212"},{"@type":"OPENAIRE","@value":"doi_dedup___::1d38957028f58d3544de2f9dbf080e43"},{"@type":"CROSSREF","@value":"10.1002/adfm.202316500_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1016/j.joule.2021.03.001_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1039/d0ee01845g_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1002/adfm.202106560_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1007/s40820-022-00842-4_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1002/adfm.202204594_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1002/smtd.202000507_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1039/d2ee01801b_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1002/solr.202300580_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1002/solr.202300253_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1038/s41467-020-16561-6_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1039/d0ee02017f_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1021/acsami.1c11683_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1002/cssc.202101573_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1002/adma.202414576_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1039/c9ta13159k_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"},{"@type":"CROSSREF","@value":"10.1016/j.mser.2020.100545_references_DOI_TND5oVGVDdeMt2JzUHW56qDLFCc"}]}