{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1362544419178199040.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1021/ja993181h"}},{"identifier":{"@type":"URI","@value":"https://pubs.acs.org/doi/pdf/10.1021/ja993181h"}}],"dc:title":[{"@value":"Photochromism of 1,2-Bis(2-methyl-5-phenyl-3-thienyl)perfluorocyclopentene in a Single-Crystalline Phase"}],"description":[{"notation":[{"@value":"1,2-Bis(2-methyl-5-phenyl-3-thienyl)perfluorocyclopentene (1a) and their derivatives, 1,2-bis(2-methyl-5-p-tolyl-3-thienyl)perfluorocyclopentene (2a) and 1,2-bis(2-methyl-5-p-tert-butylphenyl-3-thienyl)perfluorocyclopentene (3a), were found to undergo reversible photochromic reactions in the single-crystalline phase. Upon irradiation with 366 nm light the single crystals turned blue. The blue colored crystals returned to colorless by irradiation with visible light (λ > 480 nm). The substituents at para positions of the phenyl groups did not affect the rates of photocyclization reactions both in the single-crystalline phase and in hexane. Activation energies of the photocyclization reactions were almost zero. On the other hand, activation energies as much as 5−10 kJ mol-1 were observed in the photocycloreversion reactions in the single-crystalline phase. These values were smaller than those observed in solution, ca. 16 kJ mol-1. Slow thermal cycloreversion reaction of the closed-ring isomer (1b) was observ..."}]}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1382544419178199043","@type":"Researcher","foaf:name":[{"@value":"Masahiro Irie"}],"jpcoar:affiliationName":[{"@value":"Contribution from the Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University, and CREST, Japan Science and Technology Corporation, Hakozaki 6-10-1, Higashi-ku, Fukuoka 812-8581, Japan, and Institute of Advanced Material Study, Kyushu University, Kasugakoen 6-1, Fukuoka 816-8580, Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1382544419178199040","@type":"Researcher","foaf:name":[{"@value":"Thorsten Lifka"}],"jpcoar:affiliationName":[{"@value":"Contribution from the Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University, and CREST, Japan Science and Technology Corporation, Hakozaki 6-10-1, Higashi-ku, Fukuoka 812-8581, Japan, and Institute of Advanced Material Study, Kyushu University, Kasugakoen 6-1, Fukuoka 816-8580, Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1382544419178199042","@type":"Researcher","foaf:name":[{"@value":"Seiya Kobatake"}],"jpcoar:affiliationName":[{"@value":"Contribution from the Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University, and CREST, Japan Science and Technology Corporation, Hakozaki 6-10-1, Higashi-ku, Fukuoka 812-8581, Japan, and Institute of Advanced Material Study, Kyushu University, Kasugakoen 6-1, Fukuoka 816-8580, Japan"}]},{"@id":"https://cir.nii.ac.jp/crid/1382544419178199041","@type":"Researcher","foaf:name":[{"@value":"Nobuo Kato"}],"jpcoar:affiliationName":[{"@value":"Contribution from the Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University, and CREST, Japan Science and Technology Corporation, Hakozaki 6-10-1, Higashi-ku, Fukuoka 812-8581, Japan, and Institute of Advanced Material Study, Kyushu University, Kasugakoen 6-1, Fukuoka 816-8580, Japan"}]}],"publication":{"publicationIdentifier":[{"@type":"PISSN","@value":"00027863"},{"@type":"EISSN","@value":"15205126"}],"prism:publicationName":[{"@value":"Journal of the American Chemical Society"}],"dc:publisher":[{"@value":"American Chemical Society (ACS)"}],"prism:publicationDate":"2000-05-01","prism:volume":"122","prism:number":"20","prism:startingPage":"4871","prism:endingPage":"4876"},"reviewed":"false","url":[{"@id":"https://pubs.acs.org/doi/pdf/10.1021/ja993181h"}],"createdAt":"2002-07-26","modifiedAt":"2021-09-23","relatedProduct":[{"@id":"https://cir.nii.ac.jp/crid/1050022476722765696","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["isReferencedBy"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Photoluminescence ON/OFF Switching of CdSe/ZnS Core/Shell Quantum Dots Coated with Diarylethene Ligands"}]},{"@id":"https://cir.nii.ac.jp/crid/1050022476722810496","@type":"Article","resourceType":"学術雑誌論文(journal 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