The Barbier-Type Alkylation of Aldehydes with Alkyl Halides in the Presence of Metallic Strontium

  • Miyoshi Norikazu
    Department of Chemistry, Faculty of Integrated Arts and Sciences, University of Tokushima
  • Kamiura Koji
    Department of Chemistry, Faculty of Integrated Arts and Sciences, University of Tokushima
  • Oka Hiromi
    Department of Chemistry, Faculty of Integrated Arts and Sciences, University of Tokushima
  • Kita Akiko
    Department of Chemistry, Faculty of Integrated Arts and Sciences, University of Tokushima
  • Kuwata Rika
    Department of Chemistry, Faculty of Integrated Arts and Sciences, University of Tokushima
  • Ikehara Daitetsu
    Department of Chemistry, Faculty of Integrated Arts and Sciences, University of Tokushima
  • Wada Makoto
    Department of Chemistry, Faculty of Integrated Arts and Sciences, University of Tokushima

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Other Title
  • Barbier Type Alkylation of Aldehydes with Alkyl Halides in the Presence of Metallic Strontium

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Abstract

In the presence of metallic strontium, the Barbier-type alkylation of aldehydes with alkyl iodides proceeded smoothly at −15 °C under an argon atmosphere to afford the corresponding alkylated alcohols in moderate to good yields. The unusual addition reaction of ethyl benzoate with tert-butyl iodide took place to give the p-tert-butylated alkylated product (the 1,6-adduct of the benzoate) in 55% yield. Using strontium isopropoxide, the Meerwein–Ponndorf–Verley-type reduction of the aldehyde proceeded smoothly under reflux conditions in 2-propanol.

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Details

  • CRID
    1390001204128909440
  • NII Article ID
    130004151658
    10012095036
  • NII Book ID
    AA00580132
  • DOI
    10.1246/bcsj.77.341
  • ISSN
    13480634
    00092673
  • NDL BIB ID
    6845617
  • Text Lang
    en
  • Data Source
    • JaLC
    • NDL
    • Crossref
    • CiNii Articles
  • Abstract License Flag
    Disallowed

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