{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1390282679545768192.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.1252/jcej.39.216"}},{"identifier":{"@type":"NDL_BIB_ID","@value":"7873399"}},{"identifier":{"@type":"URI","@value":"http://id.ndl.go.jp/bib/7873399"}},{"identifier":{"@type":"URI","@value":"https://ndlsearch.ndl.go.jp/books/R000000004-I7873399"}},{"identifier":{"@type":"URI","@value":"http://www.jstage.jst.go.jp/article/jcej/39/2/39_2_216/_pdf"}},{"identifier":{"@type":"NAID","@value":"130000019251"}}],"dc:title":[{"@language":"en","@value":"Hydrogen Production from Ethanol Using a Plasma Reactor with an Alumite Catalyst Electrode"}],"dc:language":"en","description":[{"type":"abstract","notation":[{"@language":"en","@value":"With the aim of developing a non-equilibrium reactor for proton exchange membrane fuel cell (PEMFC) systems and other applications, hydrogen was produced from ethanol using a non-equilibrium plasma reactor combined with a catalyst, which consisted of an alumite catalyst electrode, at atmospheric pressure in a temperature range of 160–300°C under an AC or a pulsed discharge condition.<BR>It was found that non-equilibrium plasma and a catalyst had a synergistic effect on the ethanol conversion rate under an AC discharge. For example, the ethanol conversion rate obtained with the plasma reactor with the alumite catalyst (Cu-Ni/<I>γ</I>-Al<SUB>2</SUB>O<SUB>3</SUB>) electrode under an AC discharge condition of 3 kV of effective voltage at 2 kHz was 2.4 times as large as the arithmetic sum of the ethanol conversion rate obtained with the plasma reactor with a non-catalytic alumite electrode under the same discharge conditions and the ethanol conversion rate obtained with the alumite catalyst (Cu-Ni/<I>γ</I>-Al<SUB>2</SUB>O<SUB>3</SUB>) electrode without any discharge, at 210°C. It was also observed that non-equilibrium plasma and a catalyst had a synergistic effect on the ethanol conversion rate under a pulsed discharge. For example, the ethanol conversion rate obtained with the plasma reactor with the alumite catalyst (Cu-Ni/<I>γ</I>-Al<SUB>2</SUB>O<SUB>3</SUB>) electrode under a pulsed discharge of 7.2 kV of peak-to-peak voltage at a pulse number of 5000 s<SUP>–1</SUP> was 1.9 times as large as the arithmetic sum of the ethanol conversion rate obtained with the plasma reactor with the non-catalytic alumite electrode under the same discharge conditions and the ethanol conversion rate obtained with the alumite catalyst (Cu-Ni/<I>γ</I>-Al<SUB>2</SUB>O<SUB>3</SUB>) electrode without any discharge, at 180°C.<BR>The energy efficiency, which was defined as mols of hydrogen produced per unit electric power consumption, obtained with the alumite catalyst (Cu-Ni/<I>γ</I>-Al<SUB>2</SUB>O<SUB>3</SUB>) electrode at 270°C under conditions of an AC discharge of 3 kV of effective voltage at 2 kHz was 2.9 times higher than that obtained with the non-catalytic alumite electrode at 270°C under the same discharge conditions. The energy efficiency obtained with the alumite catalyst (Cu-Ni/<I>γ</I>-Al<SUB>2</SUB>O<SUB>3</SUB>) electrode at 270°C under conditions of a pulsed discharge, pulse number of 5000 s<SUP>–1</SUP> and peak-to-peak voltage of 7.2 kV was 2.6 times higher than that obtained with the non-catalytic alumite electrode at 270°C under the same discharge conditions. And the energy efficiency obtained with the alumite catalyst (Cu-Ni/<I>γ</I>-Al<SUB>2</SUB>O<SUB>3</SUB>) electrode at 270°C under conditions of a pulsed discharge, pulse number of 5000 s<SUP>–1</SUP> and peak-to-peak voltage of 7.2 kV was 2.7 times higher than that obtained under conditions of an AC discharge, frequency of 2 kHz and effective voltage of 3 kV.<BR>The energy efficiency and the conversion rate increased greatly because of the collaborative activity of the catalyst and non-equilibrium plasma. These results indicate the potential for developing a non-equilibrium reactor using an alumite catalyst electrode."}],"abstractLicenseFlag":"disallow"}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1410282679545164289","@type":"Researcher","personIdentifier":[{"@type":"NRID","@value":"9000001772094"}],"foaf:name":[{"@language":"en","@value":"Iwasaki Yasukazu"}],"jpcoar:affiliationName":[{"@language":"en","@value":"Technology Research Laboratory No. 3, Nissan Research Center, Nissan Motor Co., Ltd."}]},{"@id":"https://cir.nii.ac.jp/crid/1410282679545768322","@type":"Researcher","personIdentifier":[{"@type":"NRID","@value":"9000007024644"}],"foaf:name":[{"@language":"en","@value":"Liu Junqiang"}],"jpcoar:affiliationName":[{"@language":"en","@value":"Department of Chemical Engineering, Tokyo University of Agriculture and 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