{"@context":{"@vocab":"https://cir.nii.ac.jp/schema/1.0/","rdfs":"http://www.w3.org/2000/01/rdf-schema#","dc":"http://purl.org/dc/elements/1.1/","dcterms":"http://purl.org/dc/terms/","foaf":"http://xmlns.com/foaf/0.1/","prism":"http://prismstandard.org/namespaces/basic/2.0/","cinii":"http://ci.nii.ac.jp/ns/1.0/","datacite":"https://schema.datacite.org/meta/kernel-4/","ndl":"http://ndl.go.jp/dcndl/terms/","jpcoar":"https://github.com/JPCOAR/schema/blob/master/2.0/"},"@id":"https://cir.nii.ac.jp/crid/1390282763121208960.json","@type":"Article","productIdentifier":[{"identifier":{"@type":"DOI","@value":"10.2343/geochemj.2.0542"}},{"identifier":{"@type":"NDL_BIB_ID","@value":"029672868"}},{"identifier":{"@type":"URI","@value":"http://id.ndl.go.jp/bib/029672868"}},{"identifier":{"@type":"URI","@value":"https://ndlsearch.ndl.go.jp/books/R000000004-I029672868"}},{"identifier":{"@type":"URI","@value":"https://www.jstage.jst.go.jp/article/geochemj/53/2/53_2.0542/_pdf"}},{"identifier":{"@type":"NAID","@value":"130007624432"}}],"resourceType":"学術雑誌論文(journal article)","dc:title":[{"@language":"en","@value":"Radioactive <sup>35</sup>S emitted from the Fukushima Nuclear Power Plant and its re-suspension from the contaminated area"},{"@value":"Radioactive ³⁵S emitted from the Fukushima Nuclear Power Plant and its re-suspension from the contaminated area"}],"dc:language":"en","description":[{"type":"abstract","notation":[{"@language":"en","@value":"<p>We present a numerical study conducted using a regional Lagrangian model to account for the transport, deposition and radioactive decay of <sup>35</sup>S in sulfur dioxide and sulfate aerosols emitted into the atmosphere during the Fukushima Dai-ichi Nuclear Power Plant incident. The model is a Eulerian-Lagrangian hybrid system that accounts for chemical conversion of SO<sub>2</sub> into SO<sub>4</sub><sup>2−</sup> in a Eulerian manner. The simulations were compared to field measurements of atmospheric <sup>35</sup>S in sulfate collected at Kawamata, Tsukuba, Kashiwa, Fuchu and Yokohama, Japan. The <sup>35</sup>S emission scenario that best replicated the field measurements followed the same temporal variation pattern as the <sup>134/137</sup>Cs emissions. These results suggest that <sup>35</sup>S and <sup>134/137</sup>Cs follow a similar release pattern. Among the considered emission scenarios, a maximum flux of emitted chemical compounds was assumed to be either 100% <sup>35</sup>SO<sub>4</sub><sup>2−</sup> or 100% <sup>35</sup>SO<sub>2</sub>, with values of 4.0 × 10<sup>19</sup> molecules/hour and 4.0 × 10<sup>20</sup> molecules/hour, respectively on March 14th. These emission scenarios reflect the findings reported in the literature, where traces of <sup>35</sup>SO<sub>2</sub> were measured along with <sup>35</sup>SO<sub>4</sub><sup>2−</sup>, so the actual emission is expected to be a combination of both chemical forms. The Kawamata measurements (Figs. 5 and 6) presented a large concentration in the July–August period, several months after emissions decreased by more than an order of magnitude. To explain this anomaly, re-suspension ratios were calculated for the Kawamata site, which ranged between 0.1 and 1.5% and partially, but not fully, explain the large measured concentrations. Furthermore, they show large discrepancies with <sup>134/137</sup>Cs re-suspension values for measurements at the town of Namie. This situation indicates a lack of understanding of the transformations of <sup>35</sup>S that occurs after deposition and the mechanisms involved in the <sup>35</sup>S re-suspension process.</p>"}],"abstractLicenseFlag":"disallow"}],"creator":[{"@id":"https://cir.nii.ac.jp/crid/1410282763121208965","@type":"Researcher","personIdentifier":[{"@type":"NRID","@value":"9000402247711"}],"foaf:name":[{"@language":"en","@value":"Danielache Sebastian Oscar"}],"jpcoar:affiliationName":[{"@language":"en","@value":"Dep. of Material and Life Sciences, Faculty of Sci. & Tech., Sophia University"},{"@language":"en","@value":"Earth and Life Sci. 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J."},{"@language":"ja","@value":"Ｇｅｏｃｈｅｍ．　Ｊ．"}],"dc:publisher":[{"@language":"en","@value":"GEOCHEMICAL SOCIETY OF JAPAN"},{"@language":"ja","@value":"一般社団法人日本地球化学会"}],"prism:publicationDate":"2019","prism:volume":"53","prism:number":"2","prism:startingPage":"103","prism:endingPage":"118"},"reviewed":"false","url":[{"@id":"http://id.ndl.go.jp/bib/029672868"},{"@id":"https://ndlsearch.ndl.go.jp/books/R000000004-I029672868"},{"@id":"https://www.jstage.jst.go.jp/article/geochemj/53/2/53_2.0542/_pdf"}],"availableAt":"2019","foaf:topic":[{"@id":"https://cir.nii.ac.jp/all?q=Fukushima%20NPP","dc:title":"Fukushima NPP"},{"@id":"https://cir.nii.ac.jp/all?q=radioactive%20isotopes","dc:title":"radioactive isotopes"},{"@id":"https://cir.nii.ac.jp/all?q=35-sulfur","dc:title":"35-sulfur"},{"@id":"https://cir.nii.ac.jp/all?q=sulfur%20chemistry","dc:title":"sulfur chemistry"},{"@id":"https://cir.nii.ac.jp/all?q=Regional%20Lagrangian%20model","dc:title":"Regional Lagrangian model"}],"project":[{"@id":"https://cir.nii.ac.jp/crid/1040000781959295616","@type":"Project","projectIdentifier":[{"@type":"KAKEN","@value":"17H06105"},{"@type":"JGN","@value":"JP17H06105"},{"@type":"URI","@value":"https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-17H06105/"}],"notation":[{"@language":"ja","@value":"アイソトポログによる地球表層環境診断"},{"@language":"en","@value":"Environmental diagnosis with isotopologue tracers"}]}],"relatedProduct":[{"@id":"https://cir.nii.ac.jp/crid/1050564289060529152","@type":"Article","resourceType":"学術雑誌論文(journal article)","relationType":["references"],"jpcoar:relatedTitle":[{"@language":"en","@value":"Modeling study of long-range transport of Asian dust and anthropogenic aerosols from East Asia"},{"@value":"Modeling study of long‐range transport of Asian dust and anthropogenic aerosols from East Asia"},{"@value":"Modeling study of long-range transport of Asian dust and anthropogenic aerosols from 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