Transition-metal-free Nucleophilic 211At-astatination of Spirocyclic Aryliodonium Ylides

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Abstract

The transition-metal-free At-211-astatination of spirocyclic aryliodonium ylides via a nucleophilic aromatic substitution reaction is described. This method enables the preparation of At-211-radiolabeled compounds derived from multi-functionalized molecules and heteroarenes in good to excellent radiochemical yields.

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