Light-driven oxidation of CH_4 to C_1 chemicals catalysed by an organometallic Ru complex with O_2

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  • Nakano, Tatsuya
    Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University
  • Abe, Tsukasa
    Institute for Materials Chemistry and Engineering, Kyushu University
  • Matsumoto, Takahiro
    Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), Kyushu University Precursory Research for Embryonic Science and Technology (PRESTO), Japan Science and Technology Agency (JST)
  • Kimura, Kento
    Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University
  • Nakamura, Genta
    Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University
  • Hayami, Shinya
    Graduate School of Science and Technology, Kumamoto University
  • Shiota, Yoshihito
    Institute for Materials Chemistry and Engineering, Kyushu University
  • Yoshizawa, Kazunari
    Institute for Materials Chemistry and Engineering, Kyushu University International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), Kyushu University
  • Ogo, Seiji
    Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), Kyushu University

Bibliographic Information

Other Title
  • Light-driven oxidation of CH<sub>4</sub> to C<sub>1</sub> chemicals catalysed by an organometallic Ru complex with O<sub>2</sub>

Description

CH_4 conversion is one of the most challenging chemical reactions due to its inertness in terms of physical and chemical properties. We have achieved photo-induced C–H bond breaking of CH_4 and successive C–O bond formation to form CH_3OH concomitant with HCHO by an organometallic Ru complex with O_2.

Journal

  • RSC Advances

    RSC Advances 12 (20), 12253-12257, 2022-04-28

    Royal Society of Chemistry

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