Continuous-Flow Catalysis Using Phosphine-Metal Complexes on Porous Polymers: Designing Ligands, Pores, and Reactors

機関リポジトリ (HANDLE) オープンアクセス
  • 松本, 光
    九州大学大学院工学研究院化学工学部門
  • 岩井, 智弘
    東京大学大学院総合文化研究科広域科学専攻
  • 澤村, 正也
    北海道大学化学反応創成研究拠点 北海道大学大学院理学研究院化学部門
  • 三浦, 佳子
    Department of Chemical Engineering, Faculty of Engineering, Kyushu University

説明

Continuous-flow syntheses using immobilized catalysts can offer efficient chemical processes with easy separation and purification. Porous polymers have gained significant interests for their applications to catalytic systems in the field of organic chemistry. The porous polymers are recognized for their large surface area, high chemical stability, facile modulation of surface chemistry, and cost-effectiveness. It is crucial to immobilize transition-metal catalysts due to their difficult separation and high toxicity. Supported phosphine ligands represent a noteworthy system for the effective immobilization of metal catalysts and modulation of catalytic properties. Researchers have been actively pursuing strategies involving phosphine-metal complexes supported on porous polymers, aiming for high activities, durabilities, selectivities, and applicability to continuous-flow systems. This review provides a concise overview of phosphine-metal complexes supported on porous polymers for continuous-flow catalytic reactions. Polymer catalysts are categorized based on pore sizes, including micro-, meso-, and macroporous polymers. The characteristics of these porous polymers are explored concerning their efficiency in immobilized catalysis and continuous-flow systems.

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詳細情報 詳細情報について

  • CRID
    1050300379701181696
  • ISSN
    21926506
  • HANDLE
    2324/7178743
  • 本文言語コード
    en
  • 資料種別
    journal article
  • データソース種別
    • IRDB

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