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Reductive C(sp^3)–C(sp^3) homo-coupling of benzyl or allyl halides with H_2 using a water-soluble electron storage catalyst
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- Yatabe, Takeshi
- Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), Kyushu University Center for Small Molecule Energy, Kyushu University
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- Futakuchi, Sayaka
- Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University
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- Miyazawa, Keishi
- Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University
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- Shimauchi, Daiki
- Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University
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- Takahashi, Yukina
- Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), Kyushu University
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- Yoon, Ki-Seok
- Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), Kyushu University Center for Small Molecule Energy, Kyushu University
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- Nakai, Hidetaka
- Department of Applied Chemistry, Faculty of Science and Engineering, Kindai University
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- Ogo, Seiji
- Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), Kyushu University Center for Small Molecule Energy, Kyushu University
Bibliographic Information
- Other Title
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- Reductive C(sp<sup>3</sup>)–C(sp<sup>3</sup>) homo-coupling of benzyl or allyl halides with H<sub>2</sub> using a water-soluble electron storage catalyst
Description
This paper reports the first example of a reductive C(sp^3)–C(sp^3) homo-coupling of benzyl/allyl halides in aqueous solution by using H_2 as an electron source {turnover numbers (TONs) = 0.5–2.3 for 12 h}. This homo-coupling reaction, promoted by visible light, is catalysed by a water-soluble electron storage catalyst (ESC). The reaction mechanism, and four requirements to make it possible, are also described.
Journal
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- RSC Advances
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RSC Advances 11 (62), 39450-39454, 2021-12-09
Royal Society of Chemistry (RSC)
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Details 詳細情報について
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- CRID
- 1050581378933644672
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- ISSN
- 20462069
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- HANDLE
- 2324/7173466
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- Text Lang
- en
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- Article Type
- journal article
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- Data Source
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- IRDB
- Crossref
- KAKEN
- OpenAIRE