Damage Management in Water-Oxidizing Catalysts: From Photosystem II to Nanosized Metal Oxides
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- Monika Fekete
- School of Chemistry and the ARC Centre of Excellence for Electromaterials Science, Monash University, Victoria 3800, Australia
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- Eva-Mari Aro
- Department of Biochemistry and Food Chemistry, University of Turku, FI-20014 Turku, Finland
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- Robert Carpentier
- Groupe de Recherche en Biologie Végétale (GRBV), Université du Québec à Trois-Rivières, C.P. 500, Trois-Rivières, Québec G9A 5H7, Canada
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- Julian J. Eaton-Rye
- Department of Biochemistry, University of Otago, P.O. Box 56, Dunedin 9054, New Zealand
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- Hiroshi Nishihara
- Department of Chemistry, School of Science, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan
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- Jian-Ren Shen
- Photosynthesis Research Center, Graduate School of Natural Science and Technology/Faculty of Science, Okayama University, Okayama 700-8530, Japan
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- Suleyman I. Allakhverdiev
- Controlled Photobiosynthesis Laboratory, Institute of Plant Physiology, Russian Academy of Sciences, Botanicheskaya Street 35, Moscow 127276, Russia
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- Leone Spiccia
- School of Chemistry and the ARC Centre of Excellence for Electromaterials Science, Monash University, Victoria 3800, Australia
説明
Current energy resources largely rely on fossil fuels that are expected to be depleted in 50–200 years. On a global scale, the intensive use of this energy source has resulted in highly detrimental effects to the environment. Hydrogen production by water splitting, with sunlight as the main energy source, is a promising way to augment the production of renewable energy; however, the development of an efficient and stable water-oxidizing catalyst remains a key task before a technological breakthrough based on water splitting can be realized. A main issue hampering the development of commercially viable, non-precious-metal-based catalysts is their susceptibility to degradation. To efficiently address this major drawback, self-healing catalysts that can repair their structure without human intervention will be necessary. In this review, we focus on water oxidation by natural and artificial Mn-, Co-, and Ni-based catalysts and then discuss the self-healing properties that contribute to sustaining their cataly...
収録刊行物
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- ACS Catalysis
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ACS Catalysis 5 (3), 1499-1512, 2015-02-04
American Chemical Society (ACS)
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詳細情報 詳細情報について
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- CRID
- 1360002216635855488
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- ISSN
- 21555435
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- データソース種別
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- Crossref
- KAKEN
- OpenAIRE