Transient Protection of Organic Azides from Click Reactions with Alkynes by Phosphazide Formation

  • Tomohiro Meguro
    Laboratory of Chemical Bioscience, Institute of Biomaterials and Bioengineering, Tokyo Medical and Dental University (TMDU), 2-3-10 Kanda-Surugadai, Chiyoda-ku, Tokyo 101-0062, Japan
  • Suguru Yoshida
    Laboratory of Chemical Bioscience, Institute of Biomaterials and Bioengineering, Tokyo Medical and Dental University (TMDU), 2-3-10 Kanda-Surugadai, Chiyoda-ku, Tokyo 101-0062, Japan
  • Kazunobu Igawa
    Institute for Materials Chemistry and Engineering, Kyushu University, 6-1 Kasuga-koen, Kasuga, Fukuoka 816-8580, Japan
  • Katsuhiko Tomooka
    Institute for Materials Chemistry and Engineering, Kyushu University, 6-1 Kasuga-koen, Kasuga, Fukuoka 816-8580, Japan
  • Takamitsu Hosoya
    Laboratory of Chemical Bioscience, Institute of Biomaterials and Bioengineering, Tokyo Medical and Dental University (TMDU), 2-3-10 Kanda-Surugadai, Chiyoda-ku, Tokyo 101-0062, Japan

書誌事項

公開日
2018-06-14
資源種別
journal article
DOI
  • 10.1021/acs.orglett.8b01692
公開者
American Chemical Society (ACS)

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説明

A method for protecting organic azides from click reactions with alkynes is reported. Treatment of azides with Amphos affords phosphazides, which are stable under click reaction conditions and are easily converted back to azides by treatment with elemental sulfur. Thus, the method allows for facile modification of azide compounds via site-selective click reactions.

収録刊行物

  • Organic Letters

    Organic Letters 20 (13), 4126-4130, 2018-06-14

    American Chemical Society (ACS)

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