Immobilization and Photocurrent Activity of a Light-Harvesting Antenna Complex II, LHCII, Isolated from a Plant on Electrodes

  • Morio Nagata
    Graduate School of Engineering, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466-8555, Japan
  • Mizuki Amano
    Graduate School of Engineering, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466-8555, Japan
  • Takashi Joke
    Graduate School of Engineering, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466-8555, Japan
  • Kaoru Fujii
    Graduate School of Engineering, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466-8555, Japan
  • Ayumi Okuda
    Graduate School of Engineering, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466-8555, Japan
  • Masaharu Kondo
    Graduate School of Engineering, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466-8555, Japan
  • Shuichi Ishigure
    Graduate School of Engineering, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466-8555, Japan
  • Takehisa Dewa
    Graduate School of Engineering, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466-8555, Japan
  • Kouji Iida
    Nagoya Municipal Industrial Research Institute, Rokuban 3-4-41, Atsuta-ku, Nagoya 456-0058, Japan
  • Francesco Secundo
    Istituto di Chimica del Riconoscimento Molecolare, CNR, Via Mario Bianco 9, 20131 Milano, Italy
  • Yutaka Amao
    Department of Applied Chemistry, Oita University, 700 Dannoharu, Oita 870-1192, Japan
  • Hideki Hashimoto
    The Institute of Integrated Advanced Research, Graduate School of Science, Osaka City University, 3-3-138 Sugimoto, Sumiyoshi-ku, Osaka 558-8585, Japan
  • Mamoru Nango
    Graduate School of Engineering, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466-8555, Japan

書誌事項

公開日
2012-01-23
資源種別
journal article
DOI
  • 10.1021/mz200163e
公開者
American Chemical Society (ACS)

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説明

A light-harvesting (LH) antenna complex II, LHCII, isolated from spinach was immobilized onto an indium tin oxide (ITO) electrode with dot patterning of 3-aminopropyltriethoxysilane (APS) by utilizing electrostatic interactions between the cationic surface of the electrode and the anionic surface of stromal side of the LHCII polypeptide. Interestingly, the illumination of LHCII assembled onto the ITO electrode produced a photocurrent response that depends on the wavelength of the excitation light. Further, LHCII was immobilized onto a TiO2 nanostructured film to extend for the development of a dye-sensitized biosolar cell system. The photocurrent measured in the iodide/tri-iodide redox system of an ionic liquid based electrolyte on the TiO2 system showed remarkable enhancement of the conversion efficiency, as compared to that on the ITO electrode.

収録刊行物

  • ACS Macro Letters

    ACS Macro Letters 1 (2), 296-299, 2012-01-23

    American Chemical Society (ACS)

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