Sequential Chemical Separation of Cr and Ti from a Single Digest for High‐Precision Isotope Measurements of Planetary Materials

  • Yuki Hibiya
    Department of Earth and Planetary Science University of Tokyo Hongo 7‐3‐1 Bunkyo Tokyo 113‐0033 Japan
  • Tsuyoshi Iizuka
    Department of Earth and Planetary Science University of Tokyo Hongo 7‐3‐1 Bunkyo Tokyo 113‐0033 Japan
  • Katsuyuki Yamashita
    Graduate School of Natural Science and Technology Okayama University Okayama 700‐8530 Japan
  • Shigekazu Yoneda
    Department of Science and Engineering National Museum of Nature and Science Tsukuba 305‐0005 Japan
  • Akane Yamakawa
    National Institute for Environmental Studies (NIES) 16‐2 Onogawa Tsukuba 305‐8506 Japan

書誌事項

公開日
2018-12-21
資源種別
journal article
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1111/ggr.12249
公開者
Wiley

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説明

<jats:p>Combined determination of Cr and Ti isotopes of planetary materials offers a means with which to investigate their genetic relationship and the evolution of the protoplanetary disk. Here, we report the new sequential chemical separation procedure for combined Cr and Ti isotope ratio measurements. It comprises three steps: (a) Fe removal using <jats:styled-content style="fixed-case">AG</jats:styled-content>1‐X8 anion exchange resin, (b) Ti separation using <jats:styled-content style="fixed-case">TODGA</jats:styled-content> resin and (c) Cr separation using <jats:styled-content style="fixed-case">AG</jats:styled-content>50W‐X8 cation exchange resin (with one additional step of Ti purification using <jats:styled-content style="fixed-case">AG</jats:styled-content>1‐X8 anion exchange resin for samples having high Cr/Ti and Ca/Ti ratios). We applied the proposed procedure to terrestrial and meteorite samples with various compositions. Typical recovery rates of 90–100% were achieved with total procedural Cr and Ti blanks of 3–5 and 2–3 ng, respectively. We measured the Cr and Ti isotope compositions of the separated samples using thermal ionisation mass spectrometry and multiple collector‐inductively coupled plasma‐mass spectrometry, respectively. Our Cr and Ti isotope data were found to be consistent with those of previous studies of individual Cr and Ti isotopic compositions of the meteorites. These results demonstrate the capability of our separation method when applied to combined high‐precision Cr and Ti isotope analyses for single digests of planetary materials.</jats:p>

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