Reversible charge storage of ferrocene-adsorbed activated carbon using ionic liquid electrolytes

書誌事項

公開日
2020-09
権利情報
  • https://www.elsevier.com/tdm/userlicense/1.0/
  • https://www.elsevier.com/legal/tdmrep-license
  • https://doi.org/10.15223/policy-017
  • https://doi.org/10.15223/policy-037
  • https://doi.org/10.15223/policy-012
  • https://doi.org/10.15223/policy-029
  • https://doi.org/10.15223/policy-004
DOI
  • 10.1016/j.cplett.2020.137795
公開者
Elsevier BV

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説明

Abstract Ferrocene (FeCp2) is adsorbed within the pores of activated carbon (AC) in the gas phase. A large AC/FeCp2 contact interface enables fast charging and discharging of the resulting AC/FeCp2 hybrids at as high as 3.6–4.0 V vs. Li/Li+ by using ionic liquid electrolytes. Meanwhile, aqueous and organic electrolytes induce desorption of the adsorbed FeCp2 upon electrolyte impregnation. A charging (i.e., oxidation) process of the hybrids also accelerates the desorption because the resulting ferrocenium ion (FeCp2+) is pulled to an oppositely (i.e., negatively) charged counter electrode. Ionic liquids shield such attractive forces and prevent desorption of FeCp2.

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