Building a Bridge from Papermaking to Solar Fuels

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  • Zaiyong Jiang
    State Key Laboratory of Biobased Material and Green Papermaking Qilu University of Technology Shandong Academy of Sciences Jinan 250353 P. R. China
  • Xinhan Zhang
    State Key Laboratory of Biobased Material and Green Papermaking Qilu University of Technology Shandong Academy of Sciences Jinan 250353 P. R. China
  • Wei Sun
    Department of Chemistry University of Toronto 80 St. George St. Toronto Ontario M5S 3H6 Canada
  • Deren Yang
    State Key Laboratory of Silicon Materials School of Materials Science and Engineering Zhejiang University Hangzhou Zhejiang 310027 P. R. China
  • Paul N. Duchesne
    Department of Chemistry University of Toronto 80 St. George St. Toronto Ontario M5S 3H6 Canada
  • Yugang Gao
    State Key Lab of Crystal Materials Shandong University Jinan 250100 China
  • Zeyan Wang
    State Key Lab of Crystal Materials Shandong University Jinan 250100 China
  • Tingjiang Yan
    Department of Chemistry University of Toronto 80 St. George St. Toronto Ontario M5S 3H6 Canada
  • Zhimin Yuan
    State Key Laboratory of Biobased Material and Green Papermaking Qilu University of Technology Shandong Academy of Sciences Jinan 250353 P. R. China
  • Guihua Yang
    State Key Laboratory of Biobased Material and Green Papermaking Qilu University of Technology Shandong Academy of Sciences Jinan 250353 P. R. China
  • Xingxiang Ji
    State Key Laboratory of Biobased Material and Green Papermaking Qilu University of Technology Shandong Academy of Sciences Jinan 250353 P. R. China
  • Jiachuan Chen
    State Key Laboratory of Biobased Material and Green Papermaking Qilu University of Technology Shandong Academy of Sciences Jinan 250353 P. R. China
  • Baibiao Huang
    State Key Lab of Crystal Materials Shandong University Jinan 250100 China
  • Geoffrey A. Ozin
    Department of Chemistry University of Toronto 80 St. George St. Toronto Ontario M5S 3H6 Canada

書誌事項

公開日
2019-09-03
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/anie.201909222
公開者
Wiley

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説明

<jats:title>Abstract</jats:title><jats:p>Black liquor, an industrial waste product of papermaking, is primarily used as a low‐grade combustible energy source. Despite its high lignin content, the potential utility of black liquor as a feedstock in products manufacturing, remains to be exploited. Demonstrated here in is the use of black liquor as a primary feed‐stock for synthesizing graphene quantum dots that exhibit both up‐conversion and photoluminescence when excited using visible/near‐infrared radiation, thereby enabling the photosensitization of ultraviolet‐absorbing TiO<jats:sub>2</jats:sub> nanosheets. In addition, these graphene quantum dots can trap photo‐generated electrons to realize the effective separation of electron‐hole pairs. Together, these two processes facilitate the solar‐powered generation of H<jats:sub>2</jats:sub> from H<jats:sub>2</jats:sub>O, and CO from H<jats:sub>2</jats:sub>O–CO<jats:sub>2</jats:sub>, using broadband solar radiation.</jats:p>

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