Roadmap on organic–inorganic hybrid perovskite semiconductors and devices

  • Lukas Schmidt-Mende
    Department of Physics, University of Konstanz 1 , Universitaetsstr. 10, 78457 Konstanz, Germany
  • Vladimir Dyakonov
    Experimental Physics VI, University of Würzburg 2 , Am Hubland, 97074 Würzburg, Germany
  • Selina Olthof
    Department of Chemistry, University of Cologne 3 , Greinstraße 4-6, 50939 Cologne, Germany
  • Feray Ünlü
    Department of Chemistry, University of Cologne 3 , Greinstraße 4-6, 50939 Cologne, Germany
  • Khan Moritz Trong Lê
    Department of Chemistry, University of Cologne 3 , Greinstraße 4-6, 50939 Cologne, Germany
  • Sanjay Mathur
    Department of Chemistry, University of Cologne 3 , Greinstraße 4-6, 50939 Cologne, Germany
  • Andrei D. Karabanov
    Institute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen 4 , 45141 Essen, Germany
  • Doru C. Lupascu
    Institute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen 4 , 45141 Essen, Germany
  • Laura M. Herz
    Clarendon Laboratory, Department of Physics, University of Oxford 5 , Parks Road, Oxford OX1 3PU, United Kingdom
  • Alexander Hinderhofer
    Institute of Applied Physics, University of Tübingen 7 , Auf der Morgenstelle 10, 72076 Tübingen, Germany
  • Frank Schreiber
    Institute of Applied Physics, University of Tübingen 7 , Auf der Morgenstelle 10, 72076 Tübingen, Germany
  • Alexey Chernikov
    Department of Physics, University of Regensburg 8 , 93053 Regensburg, Germany
  • David A. Egger
    Department of Physics, Technical University of Munich 10 , 85748 Garching, Germany
  • Oleksandra Shargaieva
    Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling 11 ,’ Kekulestr. 5, 12489 Berlin, Germany
  • Caterina Cocchi
    Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling 11 ,’ Kekulestr. 5, 12489 Berlin, Germany
  • Eva Unger
    Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling 11 ,’ Kekulestr. 5, 12489 Berlin, Germany
  • Michael Saliba
    Carl von Ossietzky Universität Oldenburg, Institute of Physics 12 , Carl-von-Ossietzky-Straße 9, 26129 Oldenburg, Germany
  • Mahdi Malekshahi Byranvand
    Institute for Photovoltaics (ipv), University of Stuttgart 13 , Pfaffenwaldring 47, 70569 Stuttgart, Germany and , 52425 Jülich, Germany
  • Martin Kroll
    Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP), Technische Universität Dresden 14 , 01062 Dresden, Germany
  • Frederik Nehm
    Department of Physics and Materials Science, University of Luxembourg 15 , Luxembourg, Luxembourg
  • Karl Leo
    Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP), Technische Universität Dresden 14 , 01062 Dresden, Germany
  • Alex Redinger
    Department of Physics and Materials Science, University of Luxembourg 15 , Luxembourg, Luxembourg
  • Julian Höcker
    Experimental Physics VI, University of Würzburg 2 , Am Hubland, 97074 Würzburg, Germany
  • Thomas Kirchartz
    IEK5-Photovoltaik, Forschungszentrum Jülich 16 , 52425 Jülich, Germany and , Carl-Benz-Str. 199, 47057 Duisburg, Germany
  • Jonathan Warby
    Institute of Physics and Astronomy, University of Potsdam 17 , Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
  • Emilio Gutierrez-Partida
    Institute of Physics and Astronomy, University of Potsdam 17 , Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
  • Dieter Neher
    Institute of Physics and Astronomy, University of Potsdam 17 , Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
  • Martin Stolterfoht
    Institute of Physics and Astronomy, University of Potsdam 17 , Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
  • Uli Würfel
    Freiburg Materials Research Center (FMF), University of Freiburg 18 , Stefan-Meier-Str. 21, 79104 Freiburg, Germany
  • Moritz Unmüssig
    Freiburg Materials Research Center (FMF), University of Freiburg 18 , Stefan-Meier-Str. 21, 79104 Freiburg, Germany
  • Jan Herterich
    Freiburg Materials Research Center (FMF), University of Freiburg 18 , Stefan-Meier-Str. 21, 79104 Freiburg, Germany
  • Clemens Baretzky
    Freiburg Materials Research Center (FMF), University of Freiburg 18 , Stefan-Meier-Str. 21, 79104 Freiburg, Germany
  • John Mohanraj
    Applied Functional Polymers, Macromolecular Chemistry I, University of Bayreuth 20 , 95440 Bayreuth, Germany
  • Mukundan Thelakkat
    Applied Functional Polymers, Macromolecular Chemistry I, University of Bayreuth 20 , 95440 Bayreuth, Germany
  • Clément Maheu
    Surface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt 22 , Otto-Berndt-Strasse 3, 64287 Darmstadt, Germany
  • Wolfram Jaegermann
    Surface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt 22 , Otto-Berndt-Strasse 3, 64287 Darmstadt, Germany
  • Thomas Mayer
    Surface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt 22 , Otto-Berndt-Strasse 3, 64287 Darmstadt, Germany
  • Janek Rieger
    Lehrstuhl für Festkörperphysik, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU) 23 , Staudtstr. 7, 91058 Erlangen, Germany
  • Thomas Fauster
    Lehrstuhl für Festkörperphysik, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU) 23 , Staudtstr. 7, 91058 Erlangen, Germany
  • Daniel Niesner
    Lehrstuhl für Festkörperphysik, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU) 23 , Staudtstr. 7, 91058 Erlangen, Germany
  • Fengjiu Yang
    Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group Perovskite Tandem Solar Cells 24 , 12489 Berlin, Germany
  • Steve Albrecht
    Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group Perovskite Tandem Solar Cells 24 , 12489 Berlin, Germany
  • Thomas Riedl
    Institute of Electronic Devices, University of Wuppertal 26 , 42119 Wuppertal, Germany
  • Azhar Fakharuddin
    Department of Physics, University of Konstanz 1 , Universitaetsstr. 10, 78457 Konstanz, Germany
  • Maria Vasilopoulou
    Institute of Nanoscience and Nanotechnology, National Center for Scientific Research Demokritos 28 , 15341 Agia Paraskevi, Attica, Greece
  • Yana Vaynzof
    Integrated Center for Applied Physics and Photonic Materials (IAPP) and Center for Advancing Electronics Dresden (cfaed), Technische Universität Dresden 29 , Nöthnitzer Straße 61, 01187 Dresden, Germany
  • Davide Moia
    Max Planck Institute for Solid State Research 30 , Heisenbergstrasse 1, 70569 Stuttgart, Germany
  • Joachim Maier
    Max Planck Institute for Solid State Research 30 , Heisenbergstrasse 1, 70569 Stuttgart, Germany
  • Marius Franckevičius
    Department of Molecular Compound Physics, Center for Physical Sciences and Technology 31 (FTMC), Saulėtekio Avenue 3, Vilnius LT-10257, Lithuania
  • Vidmantas Gulbinas
    Department of Molecular Compound Physics, Center for Physical Sciences and Technology 31 (FTMC), Saulėtekio Avenue 3, Vilnius LT-10257, Lithuania
  • Ross A. Kerner
    Department of Electrical Engineering, Princeton University 32 , Princeton, New Jersey 08544, USA
  • Lianfeng Zhao
    Department of Electrical Engineering, Princeton University 32 , Princeton, New Jersey 08544, USA
  • Barry P. Rand
    Department of Electrical Engineering, Princeton University 32 , Princeton, New Jersey 08544, USA
  • Nadja Glück
    Department of Chemistry, Ludwig-Maximilians-University Munich 34 , Butenandtstr. 5-13, 81377 Munich, Germany
  • Thomas Bein
    Department of Chemistry, Ludwig-Maximilians-University Munich 34 , Butenandtstr. 5-13, 81377 Munich, Germany
  • Fabio Matteocci
    CHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor 35 Vergata, Roma 00133, Italy
  • Luigi Angelo Castriotta
    CHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor 35 Vergata, Roma 00133, Italy
  • Aldo Di Carlo
    CHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor 35 Vergata, Roma 00133, Italy
  • Matthias Scheffler
    Physics Department and IRIS Adlershof, Humboldt-Universität zu Berlin 37 , Zum Großen Windkanal 2, 12489 Berlin, Germany
  • Claudia Draxl
    Physics Department and IRIS Adlershof, Humboldt-Universität zu Berlin 37 , Zum Großen Windkanal 2, 12489 Berlin, Germany

抄録

<jats:p>Metal halide perovskites are the first solution processed semiconductors that can compete in their functionality with conventional semiconductors, such as silicon. Over the past several years, perovskite semiconductors have reported breakthroughs in various optoelectronic devices, such as solar cells, photodetectors, light emitting and memory devices, and so on. Until now, perovskite semiconductors face challenges regarding their stability, reproducibility, and toxicity. In this Roadmap, we combine the expertise of chemistry, physics, and device engineering from leading experts in the perovskite research community to focus on the fundamental material properties, the fabrication methods, characterization and photophysical properties, perovskite devices, and current challenges in this field. We develop a comprehensive overview of the current state-of-the-art and offer readers an informed perspective of where this field is heading and what challenges we have to overcome to get to successful commercialization.</jats:p>

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