Globe‐trotting Hydrogens on the Surface of the Fullerene Compound C<sub>60</sub>H<sub>6</sub>(N(CH<sub>2</sub>CH<sub>2</sub>)<sub>2</sub>O)<sub>6</sub>

書誌事項

公開日
1991-10
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/anie.199113091
公開者
Wiley

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説明

<jats:p><jats:bold>The [1,5] sigmatropic migration of hydrogen in the adduct between buckminsterfullerene</jats:bold> C<jats:sub>60</jats:sub> and morpholine (Hmorph) is fast at −25°C already. Elemental analysis, thermogravimetry, IR and NMR spectroscopy, and cyclic voltammetry all support the formulation of the adduct as C<jats:sub>60</jats:sub>H<jats:sub>6</jats:sub> (morph)<jats:sub>6</jats:sub>. The amine is covalently added to six pyracylene units. The small activation barrier to the migration is astounding, especially as large changes in the C<jats:sub>60</jats:sub> framework are involved.</jats:p>

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