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Polycyclic aromatic hydrocarbons in samples of Ryugu formed in the interstellar medium
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- Sarah S. Zeichner
- Geological and Planetary Science Division, California Institute of Technology, Pasadena, CA 91125, USA.
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- José C. Aponte
- Solar System Exploration Division, NASA Goddard Space Flight Center, Greenbelt, MD 20771, USA.
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- Surjyendu Bhattacharjee
- Geological and Planetary Science Division, California Institute of Technology, Pasadena, CA 91125, USA.
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- Guannan Dong
- Geological and Planetary Science Division, California Institute of Technology, Pasadena, CA 91125, USA.
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- Amy E. Hofmann
- Geological and Planetary Science Division, California Institute of Technology, Pasadena, CA 91125, USA.
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- Jason P. Dworkin
- Solar System Exploration Division, NASA Goddard Space Flight Center, Greenbelt, MD 20771, USA.
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- Daniel P. Glavin
- Solar System Exploration Division, NASA Goddard Space Flight Center, Greenbelt, MD 20771, USA.
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- Jamie E. Elsila
- Solar System Exploration Division, NASA Goddard Space Flight Center, Greenbelt, MD 20771, USA.
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- Heather V. Graham
- Solar System Exploration Division, NASA Goddard Space Flight Center, Greenbelt, MD 20771, USA.
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- Hiroshi Naraoka
- Department of Earth and Planetary Sciences, Kyushu University, Fukuoka 819-0395, Japan.
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- Yoshinori Takano
- Biogeochemistry Research Center, Japanese Agency for Marine-Earth Science and Technology, Yokosuka, Kanagawa 237-0061, Japan.
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- Shogo Tachibana
- Department of Earth and Planetary Science, University of Tokyo, Tokyo 113-0033, Japan.
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- Allison T. Karp
- Department of Geosciences, The Pennsylvania State University, University Park, PA 16802, USA.
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- Kliti Grice
- Western Australia Organic & Isotope Geochemistry Centre, The Institute for Geoscience Research, School of Earth and Planetary Sciences, Curtin University, Perth, Western Australia 6102, Australia.
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- Alex I. Holman
- Western Australia Organic & Isotope Geochemistry Centre, The Institute for Geoscience Research, School of Earth and Planetary Sciences, Curtin University, Perth, Western Australia 6102, Australia.
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- Katherine H. Freeman
- Department of Geosciences, The Pennsylvania State University, University Park, PA 16802, USA.
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- Hisayoshi Yurimoto
- Department of Earth and Planetary Sciences, Hokkaido University, Sapporo 060-0810, Japan.
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- Tomoki Nakamura
- Department of Earth Science, Tohoku University, Sendai 980-8578, Japan.
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- Takaaki Noguchi
- Division of Earth and Planetary Sciences, Kyoto University, Kyoto 606-8502, Japan.
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- Ryuji Okazaki
- Department of Earth and Planetary Sciences, Kyushu University, Fukuoka 819-0395, Japan.
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- Hikaru Yabuta
- Department of Earth and Planetary Systems Science, Hiroshima University, Higashi-Hiroshima 739-8526, Japan.
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- Kanako Sakamoto
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Toru Yada
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Masahiro Nishimura
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Aiko Nakato
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Akiko Miyazaki
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Kasumi Yogata
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Masanao Abe
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Tatsuaki Okada
- Department of Earth and Planetary Science, University of Tokyo, Tokyo 113-0033, Japan.
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- Tomohiro Usui
- Department of Earth and Planetary Science, University of Tokyo, Tokyo 113-0033, Japan.
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- Makoto Yoshikawa
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Takanao Saiki
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Satoshi Tanaka
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Fuyuto Terui
- Department of Mechanical Engineering, Kanagawa Institute of Technology, Atsugi 243-0292, Japan.
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- Satoru Nakazawa
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Sei-ichiro Watanabe
- Graduate School of Environmental Studies, Nagoya University, Nagoya 464-8601, Japan.
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- Yuichi Tsuda
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Kenji Hamase
- Graduate School of Pharmaceutical Sciences, Kyushu University, Fukuoka 812-8582, Japan.
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- Kazuhiko Fukushima
- Graduate School of Bioagricultural Sciences, Nagoya University, Nagoya 464-8601, Japan.
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- Dan Aoki
- Graduate School of Bioagricultural Sciences, Nagoya University, Nagoya 464-8601, Japan.
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- Minako Hashiguchi
- Graduate School of Environmental Studies, Nagoya University, Nagoya 464-8601, Japan.
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- Hajime Mita
- Department of Life, Environment and Material Science, Fukuoka Institute of Technology, Fukuoka 811-0295, Japan.
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- Yoshito Chikaraishi
- Institute of Low Temperature Science, Hokkaido University, Sapporo 060-0189, Japan.
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- Naohiko Ohkouchi
- Biogeochemistry Research Center, Japanese Agency for Marine-Earth Science and Technology, Yokosuka, Kanagawa 237-0061, Japan.
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- Nanako O. Ogawa
- Biogeochemistry Research Center, Japanese Agency for Marine-Earth Science and Technology, Yokosuka, Kanagawa 237-0061, Japan.
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- Saburo Sakai
- Biogeochemistry Research Center, Japanese Agency for Marine-Earth Science and Technology, Yokosuka, Kanagawa 237-0061, Japan.
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- Eric T. Parker
- Solar System Exploration Division, NASA Goddard Space Flight Center, Greenbelt, MD 20771, USA.
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- Hannah L. McLain
- Solar System Exploration Division, NASA Goddard Space Flight Center, Greenbelt, MD 20771, USA.
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- Francois-Regis Orthous-Daunay
- Institut de Planétologie et d’Astrophysique de Grenoble, Université Grenoble Alpes, Centre National de la Recherche Scientifique, 38000 Grenoble, France.
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- Véronique Vuitton
- Institut de Planétologie et d’Astrophysique de Grenoble, Université Grenoble Alpes, Centre National de la Recherche Scientifique, 38000 Grenoble, France.
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- Cédric Wolters
- Institut de Planétologie et d’Astrophysique de Grenoble, Université Grenoble Alpes, Centre National de la Recherche Scientifique, 38000 Grenoble, France.
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- Philippe Schmitt-Kopplin
- Analytical BioGeoChemistry, Helmholtz Zentrum München, 85764 Neuherberg, Germany.
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- Norbert Hertkorn
- Analytical BioGeoChemistry, Helmholtz Zentrum München, 85764 Neuherberg, Germany.
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- Roland Thissen
- Institut de Chimie Physique, Université Paris-Saclay, Centre National de la Recherche Scientifique, 91405 Orsay, France.
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- Alexander Ruf
- Laboratoire de Physique des Interactions Ioniques et Moléculaires, Université Aix-Marseille, Centre National de la Recherche Scientifique, 13397 Marseille, France.
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- Junko Isa
- Earth-Life Science Institute, Tokyo Institute of Technology, Tokyo 1528550, Japan.
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- Yasuhiro Oba
- Institute of Low Temperature Science, Hokkaido University, Sapporo 060-0189, Japan.
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- Toshiki Koga
- Biogeochemistry Research Center, Japanese Agency for Marine-Earth Science and Technology, Yokosuka, Kanagawa 237-0061, Japan.
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- Toshihiro Yoshimura
- Biogeochemistry Research Center, Japanese Agency for Marine-Earth Science and Technology, Yokosuka, Kanagawa 237-0061, Japan.
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- Daisuke Araoka
- Geological Survey of Japan, National Institute of Advanced Industrial Science and Technology, Tsukuba, Ibaraki 305-8567, Japan.
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- Haruna Sugahara
- Institute of Space and Astronautical Science, Japan Aerospace Exploration Agency, Sagamihara 252-5210, Japan.
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- Aogu Furusho
- Graduate School of Pharmaceutical Sciences, Kyushu University, Fukuoka 819-0395, Japan.
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- Yoshihiro Furukawa
- Department of Earth Science, Tohoku University, Sendai 980-8578, Japan.
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- Junken Aoki
- Graduate School of Pharmaceutical Sciences, University of Tokyo, Tokyo 113-0033, Japan.
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- Kuniyuki Kano
- Graduate School of Pharmaceutical Sciences, University of Tokyo, Tokyo 113-0033, Japan.
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- Shin-ichiro M. Nomura
- Department of Robotics, Tohoku University, Sendai 980-8578, Japan.
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- Kazunori Sasaki
- Human Metabolome Technologies Inc., Kakuganji, Tsuruoka, Yamagata, 997-0052, Japan.
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- Hajime Sato
- Institute for Advanced Biosciences, Keio University, Kakuganji, Tsuruoka, Yamagata 997-0052, Japan.
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- Takaaki Yoshikawa
- Horiba Advanced Technologies Co. Ltd., Kisshoin, Minami-ku, Kyoto 601-8510, Japan.
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- Satoru Tanaka
- Horiba Technology Services Co. Ltd., Kisshoin, Minami-ku, Kyoto 601-8510, Japan.
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- Mayu Morita
- Horiba Technology Services Co. Ltd., Kisshoin, Minami-ku, Kyoto 601-8510, Japan.
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- Morihiko Onose
- Horiba Technology Services Co. Ltd., Kisshoin, Minami-ku, Kyoto 601-8510, Japan.
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- Fumie Kabashima
- Laboratory Equipment Corporation Japan, Tokyo 105-0014, Japan.
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- Kosuke Fujishima
- Earth-Life Science Institute, Tokyo Institute of Technology, Tokyo 1528550, Japan.
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- Tomoya Yamazaki
- Institute of Low Temperature Science, Hokkaido University, Sapporo 060-0189, Japan.
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- Yuki Kimura
- Institute of Low Temperature Science, Hokkaido University, Sapporo 060-0189, Japan.
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- John M. Eiler
- Geological and Planetary Science Division, California Institute of Technology, Pasadena, CA 91125, USA.
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Description
<jats:p> Polycyclic aromatic hydrocarbons (PAHs) contain ≲20% of the carbon in the interstellar medium. They are potentially produced in circumstellar environments (at temperatures ≳1000 kelvin), by (~10 kelvin) interstellar clouds, or by processing of carbon-rich dust grains. We report isotopic properties of PAHs extracted from samples of the asteroid Ryugu and the meteorite Murchison. The doubly- <jats:sup>13</jats:sup> C substituted compositions (Δ2× <jats:sup>13</jats:sup> C values) of the PAHs naphthalene, fluoranthene, and pyrene are 9 to 51‰ higher than values expected for a stochastic distribution of isotopes. The Δ2× <jats:sup>13</jats:sup> C values are higher than expected if the PAHs formed in a circumstellar environment, but consistent with formation in the interstellar medium. By contrast, the PAHs phenanthrene and anthracene in Ryugu samples have Δ2× <jats:sup>13</jats:sup> C values consistent with formation by higher-temperature reactions. </jats:p>
Journal
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- Science
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Science 382 (6677), 1411-1416, 2023-12-22
American Association for the Advancement of Science (AAAS)
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Keywords
Details 詳細情報について
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- CRID
- 1360302866840286080
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- ISSN
- 10959203
- 00368075
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- Article Type
- journal article
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- Data Source
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- Crossref
- KAKEN
- OpenAIRE
