Ultrafast Dynamics of Photoexcited Gold Nanostructures on Mica Substrates Probed by Transient Absorption Spectroscopy and Time-resolved X-ray Diffraction

  • Hikaru Sotome
    Department of Chemistry, Graduate School of Science, Tohoku University
  • Yosuke Azuma
    Department of Chemistry, Graduate School of Science, Tohoku University
  • Sho Asami
    Department of Chemistry, Graduate School of Science, Tohoku University
  • Shin-ichi Matsushima
    Department of Chemistry, Graduate School of Science, Tohoku University
  • Shinji Kajimoto
    Department of Chemistry, Graduate School of Science, Tohoku University
  • Hiroshi Fukumura
    Department of Chemistry, Graduate School of Science, Tohoku University

説明

<jats:title>Abstract</jats:title> <jats:p>Gold nanostructures deposited on mica were excited with 400-nm sub-ps light pulses. Sub-ps transient absorption spectroscopy showed that excited hot electrons in the gold nanostructures decayed with a time constant of 13 ps through electron–phonon coupling in the nanostructures. Sub-ps time-resolved X-ray diffraction revealed that the (0010) mica lattice constant in a 1.7 µm thick surface layer expanded with a time constant of 6 ps.</jats:p>

収録刊行物

  • Chemistry Letters

    Chemistry Letters 44 (7), 961-963, 2015-04-17

    Oxford University Press (OUP)

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