Donor-Acceptor Triads Composed of Tetrathiafulvalene and Benzoquinone Fused by Benzene-Spacers: Application to the Positive Electrode Materials for Use in Rechargeable Batteries

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  • Tomokazu Yamauchi
    Department of Applied Chemistry, Graduate School of Engineering, Ehime University, 3 Bunkyo-cho, Matsuyama, Ehime 790-8577 , Japan
  • Wataru Hirabayashi
    Department of Applied Chemistry, Graduate School of Engineering, Ehime University, 3 Bunkyo-cho, Matsuyama, Ehime 790-8577 , Japan
  • Aya Yoshimura
    Department of Applied Chemistry, Graduate School of Engineering, Ehime University, 3 Bunkyo-cho, Matsuyama, Ehime 790-8577 , Japan
  • Masaru Yao
    Research Institute of Electrochemical Energy, National Institute of Advanced Industrial Science and Technology (AIST), 1-8-31 Midorigaoka, Ikeda, Osaka 563-8577 , Japan
  • Yohji Misaki
    Department of Applied Chemistry, Graduate School of Engineering, Ehime University, 3 Bunkyo-cho, Matsuyama, Ehime 790-8577 , Japan

説明

<jats:title>Abstract</jats:title> <jats:p>Donor-acceptor triads composed of tetrathiafulvalene (TTF) and benzoquinone (BQ) fused by a benzene-spacer (3, 4) were successfully synthesized. In the cyclic voltammetry, the bis[(2-ethyl)hexylthio]-4 (4e) exhibited five-pairs of one-electron transfer waves corresponding to the formation of both reduction and oxidation states from −1 to +4. The 3/Li cell exhibited high discharge energy density exceeding 700 mWh g−1.</jats:p>

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