Synthesis and Screening of an Oroidin Library against <i>Pseudomonas aeruginosa</i> Biofilms

書誌事項

公開日
2008-05-15
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/cbic.200700774
公開者
Wiley

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説明

<jats:title>Abstract</jats:title><jats:p>A 50‐compound library based on the marine natural product oroidin was synthesized and assayed for anti‐biofilm activity against PAO1 and PA14, two strains of the medically relevant γ‐proteobacterium <jats:italic>Pseudomonas aeruginosa</jats:italic>. Through structure–activity relationship (SAR) analysis of analogues based on the oroidin template, several conclusions can be drawn as to what structural properties of the synthetic derivatives are necessary to elicit a biological response. Notably, the most active analogues identified were those that contained a 2‐aminoimidazole (2‐AI) motif and a dibrominated pyrrolecarboxamide subunit. Here we disclose the synthesis and subsequently determined biological activity of this unique class of compounds as inhibitors of biofilm formation that have no direct antibiotic effect.</jats:p>

収録刊行物

  • ChemBioChem

    ChemBioChem 9 (8), 1267-1279, 2008-05-15

    Wiley

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