Transparent Light‐Driven Hydrogel Actuator Based on Photothermal Marangoni Effect and Buoyancy Flow for Three‐Dimensional Motion

  • Deng Pan
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • Dong Wu
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • Peng‐Ju Li
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • Sheng‐Yun Ji
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • Xuan Nie
    Department of Polymer Science and Engineering University of Science and Technology of China Hefei Anhui 230026 P. R. China
  • Sheng‐Ying Fan
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • Guo‐Yang Chen
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • Chen‐Chu Zhang
    Anhui Province Key Lab of Aerospace Structural Parts Forming Technology and Equipment Institute of Industry and Equipment Technology Hefei University of Technology Hefei Anhui 230009 P. R. China
  • Chen Xin
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • Bing Xu
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • SuWan Zhu
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • Ze Cai
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • YanLei Hu
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • JiaWen Li
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China
  • JiaRu Chu
    Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision Instrumentation University of Science and Technology of China Hefei Anhui 230027 P. R. China

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<jats:title>Abstract</jats:title><jats:p>Marangoni‐effect‐driven actuators (MDAs) have the advantages of direct light‐to‐work conversion and convenient operation, which makes it widely researched in the cutting‐edge fields including robots, micromachines, and intelligent systems. However, the MDA relies on the surface tension difference and it only works on the 2D liquid–air interface. Besides, the MDAs are normally pure black due to the light‐absorption material limitation. Herein, a transparent light‐driven 3D movable actuator (LTMA) and a 3D manipulation strategy are proposed. The LTMA is composed of photothermal nanoparticles‐doped temperature‐responsive hydrogel, whose surface energy changes as the nanoparticles absorb light energy. The 3D manipulation strategy combines Marangoni effect with photothermal buoyancy flow for realizing complex self‐propellant and floating/sinking motions. The LTMA can perform more advanced tasks such as 3D obstacle avoidance and 3D sampling. Benefiting from the porous structure of hydrogel, LTMA can naturally absorb the chemical molecules for remote sampling and automated drug delivery. The light‐driven, transparent, three‐dimensionally movable, and programmable actuator has promising prospects in the field of micromachines and intelligent systems.</jats:p>

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