Porous Carbon Hosts for Lithium–Sulfur Batteries

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  • Minya Wang
    State Key Laboratory of Silicon Materials Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province, and School of Materials Science and Engineering Zhejiang University Hangzhou 310027 P. R. China
  • Xinhui Xia
    State Key Laboratory of Silicon Materials Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province, and School of Materials Science and Engineering Zhejiang University Hangzhou 310027 P. R. China
  • Yu Zhong
    State Key Laboratory of Silicon Materials Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province, and School of Materials Science and Engineering Zhejiang University Hangzhou 310027 P. R. China
  • Jianbo Wu
    Zhejiang Provincial Key Laboratory for Cutting Tools College of Physics & Electronic Engineering Taizhou University Taizhou 318000 China
  • Ruochen Xu
    State Key Laboratory of Silicon Materials Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province, and School of Materials Science and Engineering Zhejiang University Hangzhou 310027 P. R. China
  • Zhujun Yao
    State Key Laboratory of Silicon Materials Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province, and School of Materials Science and Engineering Zhejiang University Hangzhou 310027 P. R. China
  • Donghuang Wang
    State Key Laboratory of Silicon Materials Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province, and School of Materials Science and Engineering Zhejiang University Hangzhou 310027 P. R. China
  • Wangjia Tang
    State Key Laboratory of Silicon Materials Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province, and School of Materials Science and Engineering Zhejiang University Hangzhou 310027 P. R. China
  • Xiuli Wang
    State Key Laboratory of Silicon Materials Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province, and School of Materials Science and Engineering Zhejiang University Hangzhou 310027 P. R. China
  • Jiangping Tu
    State Key Laboratory of Silicon Materials Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province, and School of Materials Science and Engineering Zhejiang University Hangzhou 310027 P. R. China

書誌事項

公開日
2018-12-18
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/chem.201803153
公開者
Wiley

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説明

<jats:title>Abstract</jats:title><jats:p>Lithium–sulfur batteries (LSBs) are considered to be one of the most promising alternatives to the current lithium‐ion batteries (LIBs) to meet the increasing demand for energy storage owing to their high energy density, natural abundance, low cost, and environmental friendliness. Despite great success, LSBs still suffer from several problems, including undermined capacity arising from low utilization of sulfur, unsatisfactory rate performance and poor cycling life owing to the shuttle effect of polysulfides, and poor electrical conductivity of sulfur. Under such circumstances, the design/fabrication of porous carbon–sulfur composite cathodes is regarded as an effective solution to overcome the above problems. In this review, different synthetic methods of porous carbon hosts and their corresponding integration into carbon–sulfur cathodes are summarized. The pore formation mechanism of porous carbon hosts is also addressed. The pore size effect on electrochemical performance is highlighted and compared. The enhanced mechanism of the porous carbon host on the sulfur cathode is systematically reviewed and revealed. Finally, the combination of porous carbon hosts and high‐profile solid‐state electrolytes is demonstrated, and the challenges to realize large‐scale commercial application of porous carbon–sulfur cathodes is discussed and future trends are proposed.</jats:p>

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