All Antimony Chalcogenide Tandem Solar Cell

  • Jianwang Zhang
    Hefei National Laboratory for Physical Sciences at Microscale CAS Key Laboratory of Materials for Energy Conversion Department of Materials Science and Engineering University of Science and Technology of China No. 96 Jinzhai Road Hefei Anhui 230026 China
  • Weitao Lian
    Hefei National Laboratory for Physical Sciences at Microscale CAS Key Laboratory of Materials for Energy Conversion Department of Materials Science and Engineering University of Science and Technology of China No. 96 Jinzhai Road Hefei Anhui 230026 China
  • Yiwei Yin
    Hefei National Laboratory for Physical Sciences at Microscale CAS Key Laboratory of Materials for Energy Conversion Department of Materials Science and Engineering University of Science and Technology of China No. 96 Jinzhai Road Hefei Anhui 230026 China
  • Xiaomin Wang
    Hefei National Laboratory for Physical Sciences at Microscale CAS Key Laboratory of Materials for Energy Conversion Department of Materials Science and Engineering University of Science and Technology of China No. 96 Jinzhai Road Hefei Anhui 230026 China
  • Rongfeng Tang
    Hefei National Laboratory for Physical Sciences at Microscale CAS Key Laboratory of Materials for Energy Conversion Department of Materials Science and Engineering University of Science and Technology of China No. 96 Jinzhai Road Hefei Anhui 230026 China
  • Chen Qian
    Australian Centre for Advanced Photovoltaics School of Photovoltaic and Renewable Energy Engineering University of New South Wales Sydney New South Wales 2052 Australia
  • Xiaojing Hao
    Australian Centre for Advanced Photovoltaics School of Photovoltaic and Renewable Energy Engineering University of New South Wales Sydney New South Wales 2052 Australia
  • Changfei Zhu
    Hefei National Laboratory for Physical Sciences at Microscale CAS Key Laboratory of Materials for Energy Conversion Department of Materials Science and Engineering University of Science and Technology of China No. 96 Jinzhai Road Hefei Anhui 230026 China
  • Tao Chen
    Hefei National Laboratory for Physical Sciences at Microscale CAS Key Laboratory of Materials for Energy Conversion Department of Materials Science and Engineering University of Science and Technology of China No. 96 Jinzhai Road Hefei Anhui 230026 China

書誌事項

公開日
2020-02-25
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/solr.202000048
公開者
Wiley

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説明

<jats:sec><jats:label/><jats:p>A proof‐of‐concept tandem solar cell using Sb<jats:sub>2</jats:sub>S<jats:sub>3</jats:sub> and Sb<jats:sub>2</jats:sub>Se<jats:sub>3</jats:sub> as top and bottom cell absorber materials is demonstrated. The bandgaps of Sb<jats:sub>2</jats:sub>S<jats:sub>3</jats:sub> and Sb<jats:sub>2</jats:sub>Se<jats:sub>3</jats:sub> are 1.74 and 1.22 eV, perfectly satisfying the requirement of tandem solar cells. The application of few‐layer graphene enables high transmittance and excellent interfacial contact in the top subcell. By controlling the thickness of the top cell for maximizing the spectral application, the tandem device delivers a power conversion efficiency of 7.93%, which outperforms the individually optimized top cell (5.58%) and bottom cell (6.50%). Mechanistical investigation shows that the tandem device is able to make up voltage loss in the subcells, which is a critical concern in the current antimony chalcogenide solar cells. This study provides an alternative approach to enhancing the energy conversion efficiency of antimony selenosulfide.</jats:p></jats:sec>

収録刊行物

  • Solar RRL

    Solar RRL 4 (4), 2020-02-25

    Wiley

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