Decarbonylative Methylation of Aromatic Esters by a Nickel Catalyst

  • Toshimasa Okita
    Department of Applied Chemistry, Waseda University, 3-4-1 Ohkubo, Shinjuku, Tokyo 169-8555, Japan
  • Kei Muto
    Department of Applied Chemistry, Waseda University, 3-4-1 Ohkubo, Shinjuku, Tokyo 169-8555, Japan
  • Junichiro Yamaguchi
    Department of Applied Chemistry, Waseda University, 3-4-1 Ohkubo, Shinjuku, Tokyo 169-8555, Japan

書誌事項

公開日
2018-05-08
資源種別
journal article
DOI
  • 10.1021/acs.orglett.8b01233
公開者
American Chemical Society (ACS)

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説明

A Ni-catalyzed decarbonylative methylation of aromatic esters was achieved using methylaluminums as methylating agents. Dimethylaluminum chlorides uniquely worked as the methyl source. Because of the Lewis acidity of aluminum reagents, less reactive alkyl esters could also undergo the present methylation. By controlling the Lewis acidity of aluminum reagents, a chemoselective decarbonylative cross-coupling between alkyl esters and phenyl esters was successful.

収録刊行物

  • Organic Letters

    Organic Letters 20 (10), 3132-3135, 2018-05-08

    American Chemical Society (ACS)

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