Quantitative Mechanochemical Methanation of CO2 with H2O in a Stainless Steel Ball Mill

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  • Yoshinari Sawama
    Laboratory of Organic Chemistry, Gifu Pharmaceutical University, 1-25-4 Daigaku-nishi, Gifu 501-1196 , Japan
  • Miki Niikawa
    Laboratory of Organic Chemistry, Gifu Pharmaceutical University, 1-25-4 Daigaku-nishi, Gifu 501-1196 , Japan
  • Kazuho Ban
    Laboratory of Organic Chemistry, Gifu Pharmaceutical University, 1-25-4 Daigaku-nishi, Gifu 501-1196 , Japan
  • Kwihwan Park
    Laboratory of Organic Chemistry, Gifu Pharmaceutical University, 1-25-4 Daigaku-nishi, Gifu 501-1196 , Japan
  • Shin-yo Aibara
    Laboratory of Organic Chemistry, Gifu Pharmaceutical University, 1-25-4 Daigaku-nishi, Gifu 501-1196 , Japan
  • Miki Itoh
    Procurement Quality Management Center, Canon Inc., 3-16-1 Shimonoge, Takatsu-ku, Kawasaki, Kanagawa 146-8501 , Japan
  • Hironao Sajiki
    Laboratory of Organic Chemistry, Gifu Pharmaceutical University, 1-25-4 Daigaku-nishi, Gifu 501-1196 , Japan

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<jats:title>Abstract</jats:title> <jats:p>Herein, we achieved nearly quantitative and selective mechanochemical conversion of CO2 to CH4 in the presence of H2O mediated by collision and friction of stainless steel balls without external heating, revealing that this conversion involves the formation of metal carbonates and hydrogenation by H2 gas in situ generated from H2O.</jats:p>

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