Photophysics of trans-stilbene analogues: Indolo[3,2-b]indole and its heterosubstituted sulfur and selenium derivatives

書誌事項

公開日
1997-03
権利情報
  • https://www.elsevier.com/tdm/userlicense/1.0/
DOI
  • 10.1016/s0301-0104(97)00018-9
公開者
Elsevier BV

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説明

Abstract The rates of radiative and nonradiative depopulation channels of the lowest excited singlet and triplet states have been determined for indolo[3,2- b ]indole and its derivatives in which one or two nitrogen atoms have been replaced by sulfur or selenium. Introduction of the heavy atom leads to activation of both S 0 ← S 1 internal conversion and T 1 ← S 1 intersystem crossing. The nonradiative rates of T 1 depopulation are affected much more strongly than the radiative ones. The results are interpreted in terms of a trans -stilbene-like character of excited indoloindoles containing heavy heteroatoms. The evidence for the geometry change upon excitation is also provided by the results of luminescence anisotropy measurements.

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