High-entropy nanoparticles: Synthesis-structure-property relationships and data-driven discovery

  • Yonggang Yao
    Department of Materials Science and Engineering, University of Maryland, College Park, MD 20742, USA.
  • Qi Dong
    Department of Materials Science and Engineering, University of Maryland, College Park, MD 20742, USA.
  • Alexandra Brozena
    Department of Materials Science and Engineering, University of Maryland, College Park, MD 20742, USA.
  • Jian Luo
    Department of NanoEngineering, Program of Materials Science and Engineering, University of California San Diego, La Jolla, CA 92093, USA.
  • Jianwei Miao
    Department of Physics and Astronomy and California NanoSystems Institute, University of California, Los Angeles, Los Angeles, CA 90095, USA.
  • Miaofang Chi
    Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, TN 37932, USA.
  • Chao Wang
    Department of Chemical and Biomolecular Engineering, Johns Hopkins University, Baltimore, MD 21218, USA.
  • Ioannis G. Kevrekidis
    Department of Chemical and Biomolecular Engineering, Johns Hopkins University, Baltimore, MD 21218, USA.
  • Zhiyong Jason Ren
    Department of Civil and Environmental Engineering and Andlinger Center for Energy and the Environment, Princeton University, Princeton, NJ 08544, USA.
  • Jeffrey Greeley
    School of Chemical Engineering, Purdue University, West Lafayette, IN 47907, USA.
  • Guofeng Wang
    Department of Mechanical Engineering and Materials Science, University of Pittsburgh, Pittsburgh, PA 15261, USA.
  • Abraham Anapolsky
    Toyota Research Institute, Los Altos, CA 94022, USA.
  • Liangbing Hu
    Department of Materials Science and Engineering, University of Maryland, College Park, MD 20742, USA.

抄録

<jats:p>High-entropy nanoparticles have become a rapidly growing area of research in recent years. Because of their multielemental compositions and unique high-entropy mixing states (i.e., solid-solution) that can lead to tunable activity and enhanced stability, these nanoparticles have received notable attention for catalyst design and exploration. However, this strong potential is also accompanied by grand challenges originating from their vast compositional space and complex atomic structure, which hinder comprehensive exploration and fundamental understanding. Through a multidisciplinary view of synthesis, characterization, catalytic applications, high-throughput screening, and data-driven materials discovery, this review is dedicated to discussing the important progress of high-entropy nanoparticles and unveiling the critical needs for their future development for catalysis, energy, and sustainability applications.</jats:p>

収録刊行物

  • Science

    Science 376 (6589), 2022-04-08

    American Association for the Advancement of Science (AAAS)

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