Remote electronic effect on the N-heterocyclic carbene-catalyzed asymmetric intramolecular Stetter reaction and structural revision of products

  • Tsubasa Inokuma
    Graduate School of Pharmaceutical Sciences, Tokushima University, Shomachi, Tokushima 770-8505, Japan
  • Kohei Iritani
    Graduate School of Pharmaceutical Sciences, Tokushima University, Shomachi, Tokushima 770-8505, Japan
  • Yuki Takahara
    Graduate School of Pharmaceutical Sciences, Tokushima University, Shomachi, Tokushima 770-8505, Japan
  • Chunzhao Sun
    Graduate School of Pharmaceutical Sciences, Tokushima University, Shomachi, Tokushima 770-8505, Japan
  • Yousuke Yamaoka
    Graduate School of Pharmaceutical Sciences, Kyoto University, Yoshida, Sakyo-ku, Kyoto 606-8501, Japan
  • Satoru Kuwano
    Graduate School of Pharmaceutical Sciences, Kyoto University, Yoshida, Sakyo-ku, Kyoto 606-8501, Japan
  • Ken-ichi Yamada
    Graduate School of Pharmaceutical Sciences, Tokushima University, Shomachi, Tokushima 770-8505, Japan

説明

<jats:p>The remote electron-withdrawing substituents on the chiral N-heterocyclic carbene enhanced rate and enantioselectivity in the asymmetric intramolecular Stetter reaction. The absolute configurations of the products were revised by X-ray diffraction.</jats:p>

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