4,5,9,10‐Pyrene Diimides: A Family of Aromatic Diimides Exhibiting High Electron Mobility and Two‐Photon Excited Emission

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  • Ze‐Hua Wu
    State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Special Function Materials and Structure Design, College of Chemistry and Chemical Engineering Lanzhou University Lanzhou 730000 P. R. China
  • Zhuo‐Ting Huang
    State Key Laboratory of Silicon Materials Key Laboratory of Macromolecule Synthesis and Functionalization Department of Polymer Science and Engineering Zhejiang University Hangzhou 310027 P. R. China
  • Rui‐Xue Guo
    State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Special Function Materials and Structure Design, College of Chemistry and Chemical Engineering Lanzhou University Lanzhou 730000 P. R. China
  • Chun‐Lin Sun
    State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Special Function Materials and Structure Design, College of Chemistry and Chemical Engineering Lanzhou University Lanzhou 730000 P. R. China
  • Li‐Chuan Chen
    State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Special Function Materials and Structure Design, College of Chemistry and Chemical Engineering Lanzhou University Lanzhou 730000 P. R. China
  • Bing Sun
    State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Special Function Materials and Structure Design, College of Chemistry and Chemical Engineering Lanzhou University Lanzhou 730000 P. R. China
  • Zi‐Fa Shi
    State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Special Function Materials and Structure Design, College of Chemistry and Chemical Engineering Lanzhou University Lanzhou 730000 P. R. China
  • Xiangfeng Shao
    State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Special Function Materials and Structure Design, College of Chemistry and Chemical Engineering Lanzhou University Lanzhou 730000 P. R. China
  • Hanying Li
    State Key Laboratory of Silicon Materials Key Laboratory of Macromolecule Synthesis and Functionalization Department of Polymer Science and Engineering Zhejiang University Hangzhou 310027 P. R. China
  • Hao‐Li Zhang
    State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Special Function Materials and Structure Design, College of Chemistry and Chemical Engineering Lanzhou University Lanzhou 730000 P. R. China

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<jats:title>Abstract</jats:title><jats:p>The design and synthesis of high‐performance n‐type organic semiconductors are important for the development of future organic optoelectronics. Facile synthetic routes to reach the K‐region of pyrene and produce 4,5,9,10‐pyrene diimide (PyDI) derivatives are reported. The PyDI derivatives exhibited efficient electron transport properties, with the highest electron mobility of up to 3.08 cm<jats:sup>2</jats:sup> V<jats:sup>−1</jats:sup> s<jats:sup>−1</jats:sup>. The tert‐butyl‐substituted compounds (t‐PyDI) also showed good one‐ and two‐photon excited fluorescence properties. The PyDI derivatives are a new family of aromatic diimides that may exhibit both high electron mobility and good light‐emitting properties, thus making them excellent candidates for future optoelectronics.</jats:p>

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