Structural, Spectroscopic, and Theoretical Elucidation of a Redox-Active Pincer-Type Ancillary Applied in Catalysis

Debashis Adhikari, Susanne Mossin, Falguni Basuli, John C. Huffman, Robert K. Szilagyi, Karsten Meyer, Daniel J. Mindiola

doi:10.1021/ja7108486

Structural, Spectroscopic, and Theoretical Elucidation of a Redox-Active Pincer-Type Ancillary Applied in Catalysis

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Debashis Adhikari

Department of Chemistry and the Molecular Structure Center, Indiana University, Bloomington, Indiana 47405, Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nuremberg, Egerlandstrasse 1, Erlangen, Germany 91058, and Department of Chemistry and Biochemistry, Montana State University, Bozeman, Montana 59717
Susanne Mossin

Department of Chemistry and the Molecular Structure Center, Indiana University, Bloomington, Indiana 47405, Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nuremberg, Egerlandstrasse 1, Erlangen, Germany 91058, and Department of Chemistry and Biochemistry, Montana State University, Bozeman, Montana 59717
Falguni Basuli

Department of Chemistry and the Molecular Structure Center, Indiana University, Bloomington, Indiana 47405, Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nuremberg, Egerlandstrasse 1, Erlangen, Germany 91058, and Department of Chemistry and Biochemistry, Montana State University, Bozeman, Montana 59717
John C. Huffman

Department of Chemistry and the Molecular Structure Center, Indiana University, Bloomington, Indiana 47405, Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nuremberg, Egerlandstrasse 1, Erlangen, Germany 91058, and Department of Chemistry and Biochemistry, Montana State University, Bozeman, Montana 59717
Robert K. Szilagyi

Department of Chemistry and the Molecular Structure Center, Indiana University, Bloomington, Indiana 47405, Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nuremberg, Egerlandstrasse 1, Erlangen, Germany 91058, and Department of Chemistry and Biochemistry, Montana State University, Bozeman, Montana 59717
Karsten Meyer

Department of Chemistry and the Molecular Structure Center, Indiana University, Bloomington, Indiana 47405, Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nuremberg, Egerlandstrasse 1, Erlangen, Germany 91058, and Department of Chemistry and Biochemistry, Montana State University, Bozeman, Montana 59717
Daniel J. Mindiola

Department of Chemistry and the Molecular Structure Center, Indiana University, Bloomington, Indiana 47405, Inorganic Chemistry, Friedrich-Alexander University Erlangen-Nuremberg, Egerlandstrasse 1, Erlangen, Germany 91058, and Department of Chemistry and Biochemistry, Montana State University, Bozeman, Montana 59717