Refined potential model for atomistic simulations of ionic liquid [bmim][PF6]

  • B. L. Bhargava
    Jawaharlal Nehru Centre for Advanced Scientific Research Chemistry and Physics of Materials Unit, , Jakkur, Bangalore 560 064, India
  • S. Balasubramanian
    Jawaharlal Nehru Centre for Advanced Scientific Research Chemistry and Physics of Materials Unit, , Jakkur, Bangalore 560 064, India

書誌事項

公開日
2007-09-21
DOI
  • 10.1063/1.2772268
公開者
AIP Publishing

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説明

<jats:p>Refined parameters of an atomistic interaction potential model for the room temperature ionic liquid 1-n-butyl,3-methylimidazolium hexafluorophosphate are presented. Classical molecular dynamics simulations have been carried out to validate this fully flexible all-atom model. It predicts the density of the liquid at different temperatures between 300 and 500K within 1.4% of the experimental value. Intermolecular radial distribution functions and the spatial distribution functions obtained from the new model are in close agreement with ab initio simulations. The calculated diffusion coefficients of ions and the surface tension of the liquid agree well with experiment.</jats:p>

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