Direct and selective conversion of methanol to para-xylene over Zn ion doped ZSM-5/silicalite-1 core-shell zeolite catalyst

Koji Miyake, Yuichiro Hirota, Kaito Ono, Yoshiaki Uchida, Shunsuke Tanaka, Norikazu Nishiyama

doi:10.1016/j.jcat.2016.07.008

Direct and selective conversion of methanol to para-xylene over Zn ion doped ZSM-5/silicalite-1 core-shell zeolite catalyst

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書誌事項

公開日: 2016-10

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http://www.elsevier.com/open-access/userlicense/1.0/

DOI

10.1016/j.jcat.2016.07.008

公開者: Elsevier BV

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説明

Abstract We successfully designed Zn ion doped ZSM-5/silicalite-1 core-shell zeolite catalyst. On methanol to para -xylene (MT p X) over the core-shell catalyst, p -xylene yield was 40.7 C-mol% and para -selectivity ( para -xylene selectivity in xylene isomers) was higher than 99 C-mol%, which substantially exceeds the other results reported in the literature.