Revisiting the adsorption of copper-phthalocyanine on Au(111) including van der Waals corrections

  • Johann Lüder
    Uppsala University Department of Physics and Astronomy, , Box 516, Uppsala 75120, Sweden
  • Olle Eriksson
    Uppsala University Department of Physics and Astronomy, , Box 516, Uppsala 75120, Sweden
  • Biplab Sanyal
    Uppsala University Department of Physics and Astronomy, , Box 516, Uppsala 75120, Sweden
  • Barbara Brena
    Uppsala University Department of Physics and Astronomy, , Box 516, Uppsala 75120, Sweden

書誌事項

公開日
2014-03-28
DOI
  • 10.1063/1.4868139
公開者
AIP Publishing

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説明

<jats:p>We have studied the adsorption of copper-phthalocyanine on Au(111) by means of van der Waals corrected density functional theory using the Tkatchenko-Scheffler method. We have compared the element and site resolved adsorption distances to recent experimental normal-incident X-ray standing wave measurements. The measured adsorption distances could be reproduced within a deviation of 1% for the Cu atom, 1% for the C atoms, and 2% for the N atoms. The molecule was found to have a magnetic moment of 1 μB distributed over the Cu and the N atoms of the pyrrole ring. Simulated scanning tunnel microscopy images based on the total and on the spin-resolved differential charge densities are provided for bias voltages of −1.45 and 1.45 eV.</jats:p>

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