Synthesis of Nitrogen‐Containing Rubicene and Tetrabenzopentacene Derivatives

  • Young S. Park
    Department of Chemical Engineering and Materials Science University of California, Irvine Irvine CA 92697 USA
  • David J. Dibble
    Department of Chemical Engineering and Materials Science University of California, Irvine Irvine CA 92697 USA
  • Juhwan Kim
    Department of Chemical Engineering and Materials Science University of California, Irvine Irvine CA 92697 USA
  • Robert C. Lopez
    Department of Chemistry University of California, Irvine Irvine CA 92697 USA
  • Eriberto Vargas
    Department of Chemical Engineering and Materials Science University of California, Irvine Irvine CA 92697 USA
  • Alon A. Gorodetsky
    Department of Chemical Engineering and Materials Science University of California, Irvine Irvine CA 92697 USA

書誌事項

公開日
2016-02-02
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/anie.201510320
公開者
Wiley

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説明

<jats:title>Abstract</jats:title><jats:p>Carbon‐based materials, such as acenes, fullerenes, and graphene nanoribbons, are viewed as the potential successors to silicon in the next generation of electronics. Although a number of methodologies provide access to these materials’ all‐carbon variants, relatively fewer strategies readily furnish their nitrogen‐doped analogues. Herein, we report the rational design, preparation, and characterization of nitrogen‐containing rubicenes and tetrabenzopentacenes, which can be viewed either as acene derivatives or as molecular fragments of fullerenes and graphene nanoribbons. The reported findings may prove valuable for the development of electron transporting organic semiconductors and for the eventual construction of larger carbonaceous systems.</jats:p>

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