Vanadium‐Catalyzed Solvent‐Free Synthesis of Quaternary α‐Trifluoromethyl Nitriles by Electrophilic Trifluoromethylation

書誌事項

公開日
2014-08-21
権利情報
  • http://onlinelibrary.wiley.com/termsAndConditions#vor
DOI
  • 10.1002/anie.201406181
公開者
Wiley

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説明

<jats:title>Abstract</jats:title><jats:p>The direct electrophilic trifluoromethylation of silyl ketene imines (SKIs) with hypervalent iodine reagents leads to the formation of quaternary α‐trifluoromethyl nitriles in good yields. This new reaction has been carried out with a variety of substituted SKIs under solvent‐free conditions using a vanadium(IV) catalyst (5 mol %). The corresponding products may be transformed into useful organofluorine building blocks.</jats:p>

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