Vertical and Lateral Transport of Particulate Radiocesium off Fukushima

  • Shigeyoshi Otosaka
    Research Group for Environmental Science, Japan Atomic Energy Agency, 2-4 Shiraka-Shirane, Tokai-mura, Ibaraki 319-1195, Japan
  • Takahiro Nakanishi
    Fukushima Environmental Research Group, Japan Atomic Energy Agency, 1-29 Okitama-cho, Fukushima-shi, Fukushima 960-8034, Japan
  • Takashi Suzuki
    Research Group for Environmental Science, Japan Atomic Energy Agency, 2-4 Shiraka-Shirane, Tokai-mura, Ibaraki 319-1195, Japan
  • Yuhi Satoh
    Research Group for Environmental Science, Japan Atomic Energy Agency, 2-4 Shiraka-Shirane, Tokai-mura, Ibaraki 319-1195, Japan
  • Hisashi Narita
    School of Marine Science and Technology, Tokai University, Shimizu-ku, Shizuoka 424-8610, Japan

書誌事項

公開日
2014-10-22
権利情報
  • http://pubs.acs.org/page/policy/authorchoice_ccbyncnd_termsofuse.html
DOI
  • 10.1021/es503736d
公開者
American Chemical Society (ACS)

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説明

Transport processes of particulate radiocesium were investigated using a sediment trap deployed at about 100 km east of the Fukushima Daiichi Nuclear Power Plant. A sediment trap was installed at 873 m depth of the station (119 m above the bottom), and time-series sampling of sinking particles was carried out from August, 2011 to June, 2013. The accident-derived radiocesium was detected from sinking particles over two years after the accident. Observed 137Cs flux was highest in September 2011 (98 mBq m(-2) day(-1): decay-corrected to March 11, 2011), and decreased over time with seasonal fluctuations. Particulate fluxes of radiocesium were mainly affected by two principal processes. One was the rapid sinking of radiocesium-bound particles (moderate mode). This mode was dominant especially in the early postaccident stage, and was presumed to establish the distribution of radiocesium in the offshore seabed. Another mode was observed in winter, and secondary transport of particles attributed to turbulence near the seabed increased fluxes of particulate radiocesium (turbulence mode). Although the latter process would not drastically change the distribution of sedimentary radiocesium in the short term, attention should be paid as this key process redistributing the accident-derived radiocesium may cumulatively affect the long-term distribution.

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