Ultrafast electron diffraction imaging of bond breaking in di-ionized acetylene
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- B. Wolter
- ICFO–Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels, Barcelona, Spain.
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- M. G. Pullen
- ICFO–Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels, Barcelona, Spain.
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- A.-T. Le
- J. R. Macdonald Laboratory, Physics Department, Kansas State University, Manhattan, KS 66506-2604, USA.
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- M. Baudisch
- ICFO–Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels, Barcelona, Spain.
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- K. Doblhoff-Dier
- Leiden Institute of Chemistry, Gorlaeus Laboratories, Leiden University, Post Office Box 9502, 2300 RA Leiden, Netherlands.
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- A. Senftleben
- Universität Kassel, Institut für Physik und CINSaT, Heinrich-Plett-Str. 40, 34132 Kassel, Germany.
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- M. Hemmer
- ICFO–Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels, Barcelona, Spain.
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- C. D. Schröter
- Max-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.
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- J. Ullrich
- Max-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.
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- T. Pfeifer
- Max-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.
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- R. Moshammer
- Max-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.
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- S. Gräfe
- Institute for Physical Chemistry, Friedrich-Schiller University Jena, 07743 Jena, Germany.
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- O. Vendrell
- Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron (DESY), Centre for Ultrafast Imaging (CUI), 22607 Hamburg, Germany.
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- C. D. Lin
- J. R. Macdonald Laboratory, Physics Department, Kansas State University, Manhattan, KS 66506-2604, USA.
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- J. Biegert
- ICFO–Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels, Barcelona, Spain.
書誌事項
- 公開日
- 2016-10-21
- 権利情報
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- http://www.sciencemag.org/about/science-licenses-journal-article-reuse
- DOI
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- 10.1126/science.aah3429
- 公開者
- American Association for the Advancement of Science (AAAS)
この論文をさがす
説明
<jats:title>Acetylene's scission visualized by selfie</jats:title> <jats:p> Can molecules take pictures of themselves? That is more or less the principle underlying laser-induced electron diffraction (LIED): A laser field strips an electron from a molecule and then sends it back to report on the structure of the remaining ion. Wolter <jats:italic>et al.</jats:italic> applied this technique to acetylene to track the cleavage of its C–H bond after double ionization (see the Perspective by Ruan). They imaged the full structure of the molecule and also distinguished more rapid dissociative dynamics when it was oriented parallel rather than perpendicular to the LIED field. </jats:p> <jats:p> <jats:italic>Science</jats:italic> , this issue p. <jats:related-article xmlns:xlink="http://www.w3.org/1999/xlink" ext-link-type="doi" issue="6310" page="308" related-article-type="in-this-issue" vol="354" xlink:href="10.1126/science.aah3429">308</jats:related-article> ; see also p. <jats:related-article xmlns:xlink="http://www.w3.org/1999/xlink" ext-link-type="doi" issue="6310" page="283" related-article-type="in-this-issue" vol="354" xlink:href="10.1126/science.aai8656">283</jats:related-article> </jats:p>
収録刊行物
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- Science
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Science 354 (6310), 308-312, 2016-10-21
American Association for the Advancement of Science (AAAS)